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Variation of temporal and spatial patterns of NO_2 in Beijing using OMI and mobile DOAS 被引量:5

Variation of temporal and spatial patterns of NO_2 in Beijing using OMI and mobile DOAS
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摘要 Control policies such as "odd-and-even license plate rule" were implemented by the Chinese government to restrict traffic and suspend factory production in Beijing and neighboring cities during the Asia-Pacific Economic Cooperation summit. We use ozone monitoring instrument(OMI), mobile differential optical absorption spectroscopy(DOAS), and multi-axis differential optical absorption spectroscopy(MAX-DOAS) to measure the variation of the spatial and temporal patterns of NO2 column densities from October 24, 2014 to November 22, 2014. It is found that the NO2 column densities during the episode of control policies are significantly lower than those during other periods, and the emission flux of NO2 calculated by mobile DOAS is also lower than the results from other periods. Some daily low NO2 column densities occur with the northwest wind direction. We then compare the relationship between OMI and mobile DOAS NO2 column density observations, and the results of mobile DOAS are approximately 2.7 times larger than the OMI values. The largest discrepancy occurs in the northern part of Beijing city. In other parts, the two instruments have a better correlation coefficient(R2) of 0.61. The low NO2 column densities that occur during the episode of control policies are affected by the control policies as well as meteorological conditions. Control policies such as "odd-and-even license plate rule" were implemented by the Chinese government to restrict traffic and suspend factory production in Beijing and neighboring cities during the Asia-Pacific Economic Cooperation summit. We use ozone monitoring instrument(OMI), mobile differential optical absorption spectroscopy(DOAS), and multi-axis differential optical absorption spectroscopy(MAX-DOAS) to measure the variation of the spatial and temporal patterns of NO2 column densities from October 24, 2014 to November 22, 2014. It is found that the NO2 column densities during the episode of control policies are significantly lower than those during other periods, and the emission flux of NO2 calculated by mobile DOAS is also lower than the results from other periods. Some daily low NO2 column densities occur with the northwest wind direction. We then compare the relationship between OMI and mobile DOAS NO2 column density observations, and the results of mobile DOAS are approximately 2.7 times larger than the OMI values. The largest discrepancy occurs in the northern part of Beijing city. In other parts, the two instruments have a better correlation coefficient(R2) of 0.61. The low NO2 column densities that occur during the episode of control policies are affected by the control policies as well as meteorological conditions.
出处 《Science China Chemistry》 SCIE EI CAS CSCD 2015年第9期1367-1376,共10页 中国科学(化学英文版)
基金 supported by the National Natural Science Foundation of China(41275038) the Key Research Program of the Chinese Academy of Sciences(KJZD-EW-TZ-G06) the National High Technology Research and Development Program of China(2014AA06A508,2014AA06A511) the Scientific and Technological Project of Anhui Province(1301022083) the Special Project of Environmental Nonprofit Industry Research,China(201409006)
关键词 OMI DOAS NO2 emission flux control policies DOAS 空间利用 变异模式 时间 差分光学吸收光谱 浓度控制 NO2 中国政府
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