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Heavy-Ion Radiation Stability of Gd_2Zr_2O_7-Pyrochlore Glass-Ceramic Wasteforms Doped by Simulated Actinides

Heavy-Ion Radiation Stability of Gd_2Zr_2O_7-Pyrochlore Glass-Ceramic Wasteforms Doped by Simulated Actinides
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摘要 To research the structure radiation stability of simulated Gd2Zr2O7-pyrochlore glass-ceramic wasteforms Nd3+, Ce4+ were selected as the simulated nuclide of An3+ and An4+ radionuclides respectively. A series of compounds with the general formula Gd2-xNdxZr2-xCexO7 (0.0≤ x ≤2.0) were prepared by High-temperature sintering method at 1623 K for 48 h in air atmosphere. The heavy-ion irradiation experiments were done at room temperature and atmospheric pressure. The structure and microscopic morphology of Gd2-xNdxZr2-xCexO7 (0.0≤ x ≤2.0) glass-ceramic wasteforms before and after irradiation experiments were investigated by the X-ray diffraction and scanning electron microscopy. To research the structure radiation stability of simulated Gd2Zr2O7-pyrochlore glass-ceramic wasteforms Nd3+, Ce4+ were selected as the simulated nuclide of An3+ and An4+ radionuclides respectively. A series of compounds with the general formula Gd2-xNdxZr2-xCexO7 (0.0≤ x ≤2.0) were prepared by High-temperature sintering method at 1623 K for 48 h in air atmosphere. The heavy-ion irradiation experiments were done at room temperature and atmospheric pressure. The structure and microscopic morphology of Gd2-xNdxZr2-xCexO7 (0.0≤ x ≤2.0) glass-ceramic wasteforms before and after irradiation experiments were investigated by the X-ray diffraction and scanning electron microscopy.
出处 《矿物学报》 CAS CSCD 北大核心 2013年第S1期84-84,共1页 Acta Mineralogica Sinica
关键词 Gd2Zr2O7-pyrochlore GLASS-CERAMIC radiation stability wasteforms Gd2Zr2O7-pyrochlore glass-ceramic radiation stability wasteforms
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