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丙烷选择氧化制丙烯酸复合金属氧化物催化剂的研究进展 被引量：1

Progress on the Research of Complex Metal Oxides Catalysts for the Selective Oxidation of Propane to Acrylic Acid
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摘要 综述了丙烷选择氧化制丙烯酸的复合金属氧化物催化剂(CMO)研究进展,特别是主要金属元素的作用以及催化剂制备过程中金属原子比、混合方法、干燥方式、焙烧气氛和pH值等因素对CMO催化性能的影响,并指出了今后的研究方向。 The development of complex metal oxide catalysts (CMO) for the selective oxidation of propane to acrylic acid (AA) is reviewed in this article. Especially, the role-played by each metal element in the CMO (Mo_aV_bTe_cNb_dO_n and Mo_aV_bSb_cNb_dO_n), and the effects of metal ratio, mixing, drying, calcination atmosphere, and gas flow and pH value on the performance of the catalysts are discussed. In addition, the review prospects the direction of development in future.
作者 张铁珍 王鉴 董群 张海燕 贾云刚
机构地区 大庆石油学院化学化工学院
出处 《江苏化工》 2004年第6期16-20,52,共6页 Jiangsu Chemical Industry
基金 黑龙江省教育厅骨干教师资助项目。
关键词 复合金属氧化物 催化剂 选择氧化 丙烷 丙烯酸 complex metal oxide catalyst selective oxidation propane acrylic acid
分类号 TQ032.41 [化学工程]
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参考文献19

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同被引文献37

  • 1赵忠奎,李宗石,王桂茹,乔卫红,程侣伯.杂多酸催化剂及其在精细化学品合成中的应用[J].化学进展,2004,16(4):620-630. 被引量：66
  • 2李秀凯,雷宇,江桥,赵静,季伟捷,张志炳,陈懿.Keggin型钼钒磷杂多酸催化剂上丙烷选择氧化性能的研究[J].化学学报,2005,63(12):1049-1054. 被引量：12
  • 3李秀凯,雷宇,赵静,季伟捷,张志炳,陈懿.结构原子组成对Keggin型杂多酸铯盐上丙烷选择氧化性能的影响[J].高等学校化学学报,2005,26(9):1716-1721. 被引量：5
  • 4杨秀娟,冯汝明,李丽,季伟捷,陈懿.在复合金属氧化物催化剂上丙烷直接氧化制丙烯酸[J].化学进展,2007,19(5):643-650. 被引量：5
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  • 7Li X K, Zhao J, Ji W J, et al. Effect of vanadium substitution in the cesium salts of Keggin-type heteropoly acids on propane partial oxidation [J]. Catal., 2006, 237(1): 58-66.
  • 8Kaddouri A, Mazzocchia C, Tempesti E. The synthesis of acrolein and acrylic acid by direct propane oxidation with Ni-Mo-Te-P-O catalysts [J].Appl. Catal. A, 1999, 180(1-2): 271-275.
  • 9Botella P, Lopez Nieto J M, Solsona B, et al. The preparation, characterization, and catalytic behavior of MoVTeNbO catalysts prepared by hydrothermal synthesis [J]. Catalysis, 2002, 209(2): 445-455.
  • 10Karmakar Swati, Volpe Jr, Anthony F. Heteropoly acid supported on polyoxometallate salts and their preparation: US, 6043184[P]. 2000-05-28.

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江苏化工
2004年 第6期

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