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Third-order optical nonlinearities of Zn_(1-x)Mg_xO thin films

Third-order optical nonlinearities of Zn_(1-x)Mg_xO thin films
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摘要 The Zn1-xMgxO thin films were deposited on sapphire substrates by reactive electron beam evaporation deposition (REBED). The X-ray diffraction (XRD) measurement demonstrates that these films undergo phase transition from hexagonal to cubic with increasing the Mg concentration. Absorption coefficients at 532 nm of the samples were obtained from the absorption spectra. Using optical Kerr effect, the thirdorder susceptibilities of the ternary films over a wide range of Mg concentrations were determined. The magnitude of X^(3) of the ternary Zn1-xMgxO films is order of 10^-11 esu at λ = 532 nm. The sample with phase mixture of both hexagonal and cubic structures shows the largest third-order susceptibility. The difference observed in the magnitude of X^(3) of Zn1-xMgxO films is attributed to the different microstructures of the ternary films, such as crystalline phase separation and crystal grains that enhance stimulated scattering. The Zn1-xMgxO thin films were deposited on sapphire substrates by reactive electron beam evaporation deposition (REBED). The X-ray diffraction (XRD) measurement demonstrates that these films undergo phase transition from hexagonal to cubic with increasing the Mg concentration. Absorption coefficients at 532 nm of the samples were obtained from the absorption spectra. Using optical Kerr effect, the thirdorder susceptibilities of the ternary films over a wide range of Mg concentrations were determined. The magnitude of X^(3) of the ternary Zn1-xMgxO films is order of 10^-11 esu at λ = 532 nm. The sample with phase mixture of both hexagonal and cubic structures shows the largest third-order susceptibility. The difference observed in the magnitude of X^(3) of Zn1-xMgxO films is attributed to the different microstructures of the ternary films, such as crystalline phase separation and crystal grains that enhance stimulated scattering.
出处 《Chinese Optics Letters》 SCIE EI CAS CSCD 2005年第10期611-614,共4页 中国光学快报(英文版)
基金 This work was supported by the National Natural Sci-ence Foundation of China under Grant No. 10174064and 50472058.
关键词 ABSORPTION Concentration (process) Control nonlinearities Crystalline materials Measurements Microstructure Optical Kerr effect Phase transitions SAPPHIRE Zinc compounds Absorption Concentration (process) Control nonlinearities Crystalline materials Measurements Microstructure Optical Kerr effect Phase transitions Sapphire Zinc compounds
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  • 1C.Y. Liu,B.P. Zhang,N.T. Binh,Y. Segawa.Third-harmonic generation from ZnO films deposited by MOCVD[J].Applied Physics B.2004(1)
  • 2R. Wang,Xiaochun Wu,Bingsuo Zou,L. Wang,Sishen Xie,Jiren Xu,Wei Huang.Nonresonant optical nonlinearity of ZnO composite nanoparticles with different interfacial chemical environments[J].Material Research Innovations.1998(1)

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