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双功能有机硫脲催化剂在不对称合成中的应用 被引量：1

Application of Bifunctional Thiourea Organocatalysts in Asymmetric Synthesis
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摘要 综述了双功能有机硫脲催化剂的发现,及其在Michael加成反应、Mannich反应及其它不对称合成反应中的应用,并展望了其应用前景。 The discovery of bifunctional thiourea organocatalysts and their application in asymmetric reactions such as Michael reaction and Mannich reaction were reviewed in the paper. The application prospect of these catalysts was put forward.
作者 代佳
机构地区 中山大学药学院药物化学研究所
出处 《精细化工中间体》 CAS 2007年第5期10-12,共3页 Fine Chemical Intermediates
关键词 有机催化剂 双功能 硫脲 不对称合成 organocatalyst bifunctional thiourea asymmetric synthesis
分类号 O621.3 [理学—有机化学]
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参考文献9

  • 1Stephen J.Connon.Organocatalysis Mediated by (Thio) Urea Derivatives[J].Chem.Eur.J.,2006,12:5 418-5 427.
  • 2Okino T,Hoashi Y,Takemoto Y.Enantioselective Michael Reaction of Malonates to Nitroolefins Catalyzed by Bifunctional Organocatalysts[J].J.Am.Chem.Soc.,2003,125:12 672-12 673.
  • 3Wang J,Li H,Duan W H.Organocatalytic Asymmetric Michael Addition of 2,4-Pentandione to Nitroolefins[J].Org.Lett.,2005,7 (21):4713-4716.
  • 4Hiemstra H,Wynberg H.Addition of Aromatic Thiols to Conjugated Cycloalkenones,Catalyzed by Chiral & Hydroxy Amines.A Mechani stic Study on Homogeneous Catalytic Asymmetric Synthesis[J].J.Am.Chem.Soc.,1981,103:417-430.
  • 5Vakulya B,Varga S,Csa'mpai A,et al.Highly Enantioselective Conjugate Addition of Nitromethane to Chalcones Using Bifunctional Cinchona Organocatalysts[J].Org.Lett,2005,7(10):1 967-1 969.
  • 6Anna G.Wenzel,Eric N,et al.Asymmetric Catalytic Mannich Reactions Catalyzed by Urea Derivatives:Enantioselective Synthesis ofβ-Aryl-β-Amino Acids[J].J.Am.Chem.Soc.,2002,124,12 964-12 965.
  • 7Song J,Wang Y,Deng L.The Mannich Reaction of Malonates with Simple Imines Catalyzed by Bifunctional Cinchona Alkaloids:Enantioselective Synthesis of β-Amino Acids[J].J.Am.Chem.Soc.,2006,128:6 048-6 049.
  • 8Wang J,Li H,Zu L,et al.Chiral Binaphthyl-derived Amine-Thiourea Organocatalyst-Promoted Asymmetric Morita-Baylis-Hillman Reaction[J].Org.Lett.,2005,7 (19):4 293-4 296.
  • 9Sohtome Y,Hashimoto Y,Nagasawaa K.Guanidine-thiourea Bifunctional Organocatalyst for the Asymmetric Henry(Nitroaldol) Reaction[J].Adv.Synth.Catal.,2005,347:1 643-1 648.

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精细化工中间体
2007年 第5期

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