摘要
The effect of Zn doping on the magnetic properties of CdCr2S4 systems is studied by mean field theory and high-temperature series expansion (HTSE). The nearest neighbouring and the next-neighbouring super-exchange interactions Jl(x) and J2(x) are evaluated for the spinel system Zn, Cd1-xCr2S4 in the range 0 〈 x 〈 1. The intra-planar and the inter-planar interactions are deduced. The HTSE combined with the Padd approximant method (PA) is applied to the spinel system ZnxCdl-,Cr2S4. The magnetic phase diagram, i.e. Tc versus dilution x, is obtained. The critical exponents associated with the magnetic susceptibility 7 and the correlation length u are deduced. The obtained theoretical results are in agreement with the experimental data obtained by magnetic measurements.
The effect of Zn doping on the magnetic properties of CdCr2S4 systems is studied by mean field theory and high-temperature series expansion (HTSE). The nearest neighbouring and the next-neighbouring super-exchange interactions Jl(x) and J2(x) are evaluated for the spinel system Zn, Cd1-xCr2S4 in the range 0 〈 x 〈 1. The intra-planar and the inter-planar interactions are deduced. The HTSE combined with the Padd approximant method (PA) is applied to the spinel system ZnxCdl-,Cr2S4. The magnetic phase diagram, i.e. Tc versus dilution x, is obtained. The critical exponents associated with the magnetic susceptibility 7 and the correlation length u are deduced. The obtained theoretical results are in agreement with the experimental data obtained by magnetic measurements.