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Probing Wave Packet Dynamics of I2^- Anions with Pump-Probe Femtosecond Spectroscopy 被引量:3

Probing Wave Packet Dynamics of I2^- Anions with Pump-Probe Femtosecond Spectroscopy
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摘要 The wave packet dynamics of I2^- anions is studied by using the time-dependent wave packet method. Two conclusions can be drawn from the calculations. First, the period of the total photoelectron signal oscillating with the propagation of delay time is about 750fs. Second, the photoionization of I2^- anions begin at the time 600 fs, and the time needed for the population of the electronic state of I2 neutral molecule to reach the maximum becomes shorter with the increasing delay time. The wave packet dynamics of I2^- anions is studied by using the time-dependent wave packet method. Two conclusions can be drawn from the calculations. First, the period of the total photoelectron signal oscillating with the propagation of delay time is about 750fs. Second, the photoionization of I2^- anions begin at the time 600 fs, and the time needed for the population of the electronic state of I2 neutral molecule to reach the maximum becomes shorter with the increasing delay time.
出处 《Chinese Physics Letters》 SCIE CAS CSCD 2008年第3期915-918,共4页 中国物理快报(英文版)
基金 Supported by the National Natural Science Foundation of China under Grant No 10575017. The code used in our calculation is provided by Professor Ke-Li Han and we appreciate his help and kind advice.
关键词 RESOLVED PHOTOELECTRON-SPECTRUM PHOTODISSOCIATION DYNAMICS MULTIPHOTON IONIZATION LASER-PULSES NAI PHOTOIONIZATION DISSOCIATION STATE RESOLVED PHOTOELECTRON-SPECTRUM PHOTODISSOCIATION DYNAMICS MULTIPHOTON IONIZATION LASER-PULSES NAI PHOTOIONIZATION DISSOCIATION STATE
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