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Transient Non-Thermal Mobility of CO for CO-NO Catalytic Reaction on Square Lattice: Monte Carlo Simulation

Transient Non-Thermal Mobility of CO for CO-NO Catalytic Reaction on Square Lattice: Monte Carlo Simulation
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摘要 We study a model based on precursor mechanism for CO-NO catalytic reaction on square lattice with Monte Carlo simulation. The precursor mechanism clearly demonstrates its impact on the phase diagram. The steady reactive state (SRS) gets established. The width of reactive region increases by increasing the range of precursor mobility. When the precursor mobility is increased to third-nearest neighbourhood, the second-order transition disappears. We study a model based on precursor mechanism for CO-NO catalytic reaction on square lattice with Monte Carlo simulation. The precursor mechanism clearly demonstrates its impact on the phase diagram. The steady reactive state (SRS) gets established. The width of reactive region increases by increasing the range of precursor mobility. When the precursor mobility is increased to third-nearest neighbourhood, the second-order transition disappears.
机构地区 Department of Physics
出处 《Chinese Physics Letters》 SCIE CAS CSCD 2008年第4期1482-1485,共4页 中国物理快报(英文版)
关键词 ELEY-RIDEAL PROCESS PHASE-DIAGRAM HETEROGENEOUS CATALYSIS PRECURSOR MECHANISM HEXAGONAL SURFACES CUBIC STRUCTURE SUBSURFACE MODEL CHEMISORPTION TRANSITIONS ELEY-RIDEAL PROCESS PHASE-DIAGRAM HETEROGENEOUS CATALYSIS PRECURSOR MECHANISM HEXAGONAL SURFACES CUBIC STRUCTURE SUBSURFACE MODEL CHEMISORPTION TRANSITIONS
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