Dynamical theory of spectroscopy with femtosecond pulse excitation (Ⅰ)——Dynamics of absorption and emission processes 被引量：1

Dynamical theory of spectroscopy with femtosecond pulse excitation (Ⅰ)——Dynamics of absorption and emission processes

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摘要 A dynamical theory of spectroscopy with femtosecond pulse excitation is developed and is applied to studying the one-photon absorption and two-photon emission processes.Unlike the previous theories,this theory can treat all kinds of optical process from ultrashort pulse to CW limit in a consistent picture,because the exact equation of emission rate obtained from this theory can correctly reduce to the Kramers-Heisenberg-Dirac (KHD) expression. A dynamical theory of spectroscopy with femtosecond pulse excitation is developed and is applied to studying the one-photon absorption and two-photon emission processes.Unlike the previous theories,this theory can treat all kinds of optical process from ultrashort pulse to CW limit in a consistent picture,because the exact equation of emission rate obtained from this theory can correctly reduce to the Kramers-Heisenberg-Dirac (KHD) expression.

作者陆靖 Lee Soo-Ying 范康年

机构地区 Department of Chemistry Department of Chemistry

出处《Science China Mathematics》 SCIE 1997年第9期958-966,共9页 中国科学：数学（英文版）

关键词 FEMTOSECOND ULTRASHORT PULSE RAMAN spectroscopy. femtosecond,ultrashort pulse,Raman spectroscopy.

分类号 O433 [机械工程—光学工程]

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同被引文献13

1Jing Lu,Soo-ying Lee,Kangnian Fan.Dynamical theory of spectroscopy with femtosecond pulse excitation[J]. Science in China Series A: Mathematics . 1997 (12)
2Jing Lu,Soo-Ying Lee,Kangnian Fan.Dynamical theory of spectroscopy with femtosecond pulse excitation (I)[J]. Science in China Series A: Mathematics . 1997 (9)
3Lee S Y,Lu J.Dynamics theory of Raman scattering with pulses, In: Chergui M, ed. . 1996
4Child,M. S. Molecular Physics . 1976
5Lu,J.,Lee,Soo-Y.Theory of Raman scattering with pulses: application to continuum Raman spectroscopy. The Journal of Chemical Physics . 1996
6Blukis U,Howell J M.Computer series 38. Journal of Chemical Education . 1983
7Kolba E,Manz J,Schreier H J,et al.A reflection principle in continuum resonance scattering. Chemical Physics Letters . 1992
8Lee S Y.Derivation of the reflection principle in continuum resonance Raman scattering. Chemical Physics Letters . 1993
9Levy,L,Shapiro,M.Excitation-emission study of continuum Raman and the photofragment mapping of IBr, J. The Journal of Chemical Physics . 1992
10Kosloff R.Time-dependent quantum-mechanical methods for molecular dynamics. The Journal of Chemical Physics . 1988

引证文献1

1Jing Lu,Kangnian Fan,Soo-ying Lee.Dynamical theory of spectroscopy with pulse excitation——Application to continuum Raman of IBr[J].Chinese Science Bulletin,1999,44(2):139-142. 被引量：1

二级引证文献1

1陆靖,范康年.Dynamical theory of spectroscopy with femtosecond pulse excitation(Ⅲ)——Transient rate equation in Liouville space[J].Science China Mathematics,1999,42(6):666-672.

1陆靖,Lee Soo-ying,范康年.Dynamical theory of spectroscopy with femtosecond pulse excitation——Emission of direct dissociation[J].Science China Mathematics,1997,40(12):1331-1339. 被引量：1
2郭睿,田播,吕兴,张海强,许韬.Integrability Aspects and Soliton Solutions for a System Describing Ultrashort Pulse Propagation in an Inhomogeneous Multi-Component Medium[J].Communications in Theoretical Physics,2010(9):536-544.
3周兆妍,袁建民.Fine splits of photon emission spectrum of hydrogen atom caused by transitions between different dressed states in intense high frequency laser field[J].Chinese Physics B,2008,17(12):4523-4528.
4Qingwei Yang,Xinglong Xie,Jun Kang,Haidong Zhu,Ailin Guo,Qi Gao.Independent and continuous third-order dispersion compensation using a pair of prisms[J].High Power Laser Science and Engineering,2014,2(4):68-73.
5张开成,刘邦贵.Unified nonequilibrium dynamical theory for exchange bias and training effects[J].Chinese Physics B,2009,18(9):3960-3965.
6刘晔,周飞,张道中,李志远.Energy Squeeze of Ultrashort Light Pulse by Kerr Nonlinear Photonic Crystals[J].Chinese Physics Letters,2009,26(1):122-125.
7Jing Lu,Kangnian Fan,Soo-ying Lee.Dynamical theory of spectroscopy with pulse excitation——Application to continuum Raman of IBr[J].Chinese Science Bulletin,1999,44(2):139-142. 被引量：1
8汤宇晖,韩申生,等.Stimulated Raman backscattering from an ultrashort laser interacting with underdense plasmas[J].Chinese Physics B,2002,11(1):50-53. 被引量：1
9孔艳,陈险峰,夏宇兴.Optimized Second Harmonic Generation of Femtosecond Pulse by Phase-Blanking Effect in Aperiodically Optical Superlattice[J].Chinese Physics Letters,2008,25(4):1297-1300. 被引量：1
10廖家莉,马修·马克,贾辉,孙文超,刘菊,谭一舟,唐武胜,李修建,黄智维.Ultrashort chirped pulse evolution in silicon photonic nanowlres[J].Chinese Optics Letters,2014,12(A01):129-131.

Science China Mathematics

1997年第9期

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Dynamical theory of spectroscopy with femtosecond pulse excitation (Ⅰ)——Dynamics of absorption and emission processes 被引量：1

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