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吸附-电催化氧化降解气态氯苯 被引量:8

Degradation of gaseous chlorobenzene by adsorption-electro-catalytic oxidation methods
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摘要 采用高接触面积微孔曝气的方式,以吸附性多孔导电材料活性炭纤维(ACF)为电极,吸附-电催化氧化两步联动降解气态氯苯,实现了在电解质水溶液中对高浓度非水溶性气态挥发性有机废气的有效处理。正交实验和单因素分析实验结合,确立最佳实验条件并着重考虑pH值、鼓气速率、电解电压、电解质浓度等因素对去除率的影响。在最佳实验条件下,气相中氯苯去除率达到74.3%(20℃)和72.9%(10℃) High concentration gaseous chlorobenzene was successfully removed by adsorption-eletrochemical oxidation in aqueous environment in which activated carbon fiber electrodes and micro-aeration were employed to realize the treatment. Optimal experimental parameters were determined by orthogonal and single factor effect test, and effects of pH, aeration rate, voltage and electrolyte concentration on the experimental results were considered. Under the optimal conditions, gaseous chlorobenzene removal was 74.3% (20℃) and 72.9% ( 10℃ ).
作者 魏静 杨骥
出处 《环境工程学报》 CAS CSCD 北大核心 2009年第8期1465-1468,共4页 Chinese Journal of Environmental Engineering
基金 国家自然科学基金资助项目(20507014) 教育部归国留学基金 上海市自然科学基金(05ZR14071) 教育部新世纪优秀人才(2006)资助项目
关键词 电化学 氯苯 活性炭纤维 羟基自由基(·OH) electrochemistry chlorobenzene activated carbon fiber(ACF) hydroxyl radical
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  • 1樊奇,羌宁.挥发性有机废气净化技术研究进展[J].四川环境,2005,24(4):40-44. 被引量:56
  • 2Panizza M. , Bocca C. , Cerisola G. Electrochemical treat- ment of wastewater containing polyaromatic organic pollutants. Water Research, 2000, 34 (9) :2601- 2606.
  • 3魏守强,刘瑛,史敬伟.电化学法处理含酚模拟废水的实验研究[J].沈阳工业学院学报,2003,22(4):86-88. 被引量:4
  • 4Xu Xiangrong, Li Huabin,Wang Wenhua, et al. Degradation of dyes solutions by the Fenton process. Chemosphere, 2004,57 ( 7 ) :595- 600.
  • 5Enric Brillas, Juan Casado. Aniline degradation by electro- Fcnton and peroxi-coagulation processes using a flow reactor for wastewater treatment. Chemosphere,2002, 47:241 248.
  • 6王爱民,曲久辉,史红星,茹加,刘会娟,雷鹏举.活性碳纤维阴极电芬顿反应降解微囊藻毒素研究[J].高等学校化学学报,2005,26(9):1669-1672. 被引量:23
  • 7Ventura A. , Jacquet G. , Bermond A. , et al. Electrochemical generation of the Fenton' s reagent:Application to trazine degradation. Water Research ,2002,36:3517 - 3522.
  • 8Malik P. K. , Saha S. K. Oxidation of direct dyes with hydrogen peroxide using ferrous ion as catalyst. Separation Purification Technology, 2003,31 : 244 - 250.
  • 9Songhu Yuan, MengTian, YanpingCui, et al. Treatment of nitrophenols by cathode reduction and electro-Fenton methods. Journal of Hazardous Materials, 2006, B137:573 -580.
  • 10张云山,李日扬,吴淮,李红.电生羟基自由基在有机废水处理中的应用[J].化工时刊,2005,19(6):40-42. 被引量:10

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