期刊文献+

Characteristic of organic aerosol in a remote area of Okinawa Island 被引量:1

Characteristic of organic aerosol in a remote area of Okinawa Island
下载PDF
导出
摘要 A continuous investigation of aerosol pollutants in Cape Hedo, Japan was conducted from October 2005 to August 2006 by Aerodyne aerosol mass spectrometer (AMS). This article focused on the analysis of long-range transport of organic aerosol from continental origin to the remote island. Based on the transport distance and air mass origin, four main air mass origins were considered, including North China, South China, Japan and Korea. Although the mass concentration and air mass origin were quite different during study period, the mass spectrum and size distribution of organic matter and oxidized organics were similar, which showed uni-modal distribution with modal diameter of around 500 nm. The loss rate of organics was (5.15 ± 0.55) × 10^-6 s^-1 obtained by plotting the concentration against the transport time. Conversion rate of SO2 to sulfate and oxidation rate of organics were (1.07 ± 0.15) × 10^-5 and (1.09 ± 0.52) × 10^-6 s^-1, respectively. A continuous investigation of aerosol pollutants in Cape Hedo, Japan was conducted from October 2005 to August 2006 by Aerodyne aerosol mass spectrometer (AMS). This article focused on the analysis of long-range transport of organic aerosol from continental origin to the remote island. Based on the transport distance and air mass origin, four main air mass origins were considered, including North China, South China, Japan and Korea. Although the mass concentration and air mass origin were quite different during study period, the mass spectrum and size distribution of organic matter and oxidized organics were similar, which showed uni-modal distribution with modal diameter of around 500 nm. The loss rate of organics was (5.15 ± 0.55) × 10^-6 s^-1 obtained by plotting the concentration against the transport time. Conversion rate of SO2 to sulfate and oxidation rate of organics were (1.07 ± 0.15) × 10^-5 and (1.09 ± 0.52) × 10^-6 s^-1, respectively.
出处 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2009年第10期1371-1377,共7页 环境科学学报(英文版)
基金 supported by the Western Pacific Air-Sea Interaction Study (No W-PASS, 2006-2010) the National Natural Science Foundation of China (No 40505027) the Beijing Natural Science Foundation (No 8093035)
关键词 long-range transport OKINAWA ORGANICS loss rate long-range transport Okinawa organics loss rate
  • 相关文献

参考文献20

  • 1ADORC (Acid Deposition and Oxidant Research Center),2006.Tropospheric ozone:A growing threat.ADORC,Niigata.
  • 2Alfarra M R,Coe H,Allan J D,Bower K N,Boudries H,Canagaratna M R et al.,2004.Characterization of urban and regional organic aerosols in the Lower Fraser Valley using two Aerodyne aerosol mass spectrometers.Atmospheric Environment,38:5745-5758.
  • 3Allan J D,Jimenez J L,Coe H,Bower K N,Williams P I,Worsnop D R,2003a.Quantitative sampling using an Aerodyne aerosol mass spectrometer.Part 1:techniques of data interpretation and error analysis.Journal of Geophysical Research-Atmospheres,108(D3):4090.doi:10.1029/2002JD002358.
  • 4Allan J D,Coe H,Bower K N,Williams P I,Gallagher M W,Alfarra M R et al.,2003b.Quantitative sampling using an Aerodyne aerosol mass spectrometer.Part 2:measurements of fine particulate chemical composition in two UK cities.Journal of Geophysical Research-Atmospheres,108(D3):4091.doi:10.1029/2002JD002359.
  • 5Allan J D,Delia A E,Coe H,Bower K N,Alfarra M,Jimenez J L et al.,2004.Technical note:extraction of chemically resolved mass spectra from Aerodyne aerosol mass spectrometer data.Journal of Aerosol Science,35:909-922.
  • 6Arndt R L,Carmichael G R,1995.Long-range transport and deposition of sulfur in Asia.Water,Air,and Soil Pollution,85:2283-2288.
  • 7Calori G,Carmichael G R,Streets D,Thongboonchoo N,Guttikunda S K,2001.Interannual variability in sulfur deposition in Asia.Journal of Global Environment Engineering,7:1-16.
  • 8Carmichael G R,Peters L K,Saylor R D,1991.The STEM-Π regional scale acid deposition and photochemical oxidant model:Ι.An overview of model development and applications.Atmospheric Environment,25A:2077-2090.
  • 9Carmichael G R,Hayami H,Calori G,Uno I,Cho S Y,Engardt M et al.,2001.Model intercomparison study of long range transport and sulfur deposition in East Asia (MICS-Asia).Water,Air,and Soil Pollution,130:51-62.
  • 10DeCarlo P,Slowik J G,Worsnop D R,Davidovits P,Jimenez J L,2004.Particle morphology and density characterization by combined mobility and aerodynamic diameter measurements.Part 1:theory.Aerosol Science and Technology,38:1185-1205.

引证文献1

相关作者

内容加载中请稍等...

相关机构

内容加载中请稍等...

相关主题

内容加载中请稍等...

浏览历史

内容加载中请稍等...
;
使用帮助 返回顶部