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快速退火对Pt/BST/Pt电容器结构和性能的影响 被引量:1

Effect of rapid thermal annealing on the structure and physical properties of Pt/BST/Pt capacitors
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摘要 采用脉冲激光沉积(PLD)法在Pt/Ti/SiO2/Si(001)基片上制备了Ba0.6Sr0.4TiO3(BST)薄膜,对Pt/BST/Pt电容器在空气中进行400℃快速退火(RTA)处理,研究了快速退火对Pt/BST/Pt电容器的结构和性能的影响。结果表明:快速退火虽然对BST薄膜的结晶质量影响较小,但却极大改善了Pt/BST/Pt电容器的电学性能。当测试频率为100kHz、直流偏压为0V时,介电损耗从快速退火前的0.07减小到0.03,介电常数和调谐率略有增加。快速退火后负向漏电流过大现象得到了明显抑制,正负向漏电流趋于对称,在300×103V/cm电场强度下,漏电流密度为4.83×10–5A/cm2。 Ba0.6Sr0.4TiO3(BST) thin film was fabricated on Pt/Ti/SiO2/Si(001) substrate by the pulsed laser deposition (PLD) method. The Pt/BST/Pt capacitors were treated by rapid thermal annealing (RTA) in air at 400℃. Effects of RTA on the structure and physical properties of the Pt/BST/Pt capacitors were investigated. The results show that the microstructure of BST thin film does not change obviously after annealing, but the electrical properties of the BST capacitors are enhanced greatly. The dielectric loss of the BST capacitors, measured at 100 kHz and zero-bias voltage, is reduced from 0.07 to 0.03 after RTA, and the permittivity and tunability are also slightly increased after RTA. The negative leakage current of the BST capacitors is significantly lowered after RTA. The symmetric current characteristics at positive and negative bias voltage are obtained, and the leakage current density is 4.83×10^-5A/cm^2 at 300×10^3 V/cm.
出处 《电子元件与材料》 CAS CSCD 北大核心 2009年第12期39-42,共4页 Electronic Components And Materials
基金 国家自然科学基金资助项目(No.60876055) 河北省自然科学基金资助项目(No.E2008000620 E2009000207) 教育部科学技术研究重点资助项目(No.207013) 河北省应用基础研究计划重点基础研究资助项目(No.08965124D)
关键词 BST薄膜 快速退火 Pt/BST界面层 氧空位 脉冲激光沉积 BST thin film rapid thermal annealing Pt/BST interfacial layer oxygen vacancy pulsed laser deposition
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参考文献16

  • 1SHEN H, GAO Y H, ZHOU P, et al. Effect of oxygen to argon ratio on properties of (Ba,Sr)TiO3 thin films prepared on LaNiO3/Si substrates [J] J Appl Phys, 2009, 105(061637): 1-4.
  • 2NAGARAJ B, SAWHNEY T, PERUSSE S, et al. (Ba,Sr)TiO3 thin films with conducting perovskite electrodes for dynamic random access memory applications [J]. Appl Phys Lett, 1999, 74(21): 3194-3196.
  • 3KIM H S, HYUN T S, KIM H G, et al. Orientation effect on microwave dielectric properties of Si-integrated Ba0.6Sr0.4TiO3 thin films for frequency agile devices [J]. Appl Phys Lett, 2006, 89: 1-3.
  • 4MIAO J, CHEN W R, ZHAO L, et al. Enhanced dielectric properties of Ba1-xSrxTiO3 thin film grown on Lal-xSrxMnO3 bottom layer [J]. J Appl Phys, 2004, 96(11): 6578-6584.
  • 5SUN X H, ZHU B L, LIU T, et al. Dielectric and tunable properties of K-doped Ba0.6Sr0.4TiO3 thin films fabricated by sol-gel method [J]. J Appl Phys, 2006, 99: 1-6.
  • 6PODPIRKA A, COLE M W, RAMANATIIAN S, et al. Effect of photon irradiation on structural, dielectric, and insulating properties of Ba0.60Sr0.40TiO3 thin films [J]. J Appl Phys, 1997, 82(5): 2359-2364.
  • 7COLE M W, NGO E, HIRSCH S, et al. The fabrication and material properties of compositionally multilayered Ba1-xSrxTiO3 thin films for realization of temperature insensitive tunable phase shifter devices [J]. J Appl Phys, 2007, 102(034104): 1-11.
  • 8JOO J H, JEON Y C, SEON J M, et al. Effects of post-annealing on the conduction properties of Pt/(Ba, Sr)TiO3/Pt Capacitors [J]. Jpn J Appl Phys, 1997, 36: 4382-4385.
  • 9HWANG C S, JOO S H. Variations of the leakage current density and the dielectric constant of Pt/(Ba,Sr)TiO3/Pt capacitors by annealing under a N2 atmosphere [J]. J Appl Phys, 1999, 85(4): 2431-24366.
  • 10JOO J H, SEON J M, JEON Y C, et al. Improvement of leakage currents of Pt/(Ba, Sr)TiO3/Pt capacitors [J]. Appl Phys Lett, 1997. 70(22): 3053-3055.

同被引文献14

  • 1Dai X H, Zhao H D, Zhang L, et al. Investigation of Leakage Current Behavior of Pt/Bio.975 Lao.o25 Feo.975 Nio.o25 03/Pt Capacitor Measured at Difterent Temperatures[ J]. Surface Review anti Letters ,2014,21 ( 2 ) : 14.50029.
  • 2Yang L H, Ponchel F, Wang G S, et al. Microwave Properties of Epitaxial (111 )-oriented Bao. 6 Sr0.4 TiO3 Thin Films 'on A12 03 (0001) up to 40 GHz [ J ]. Appl. Phys. Lett. ,2010,97 : 162909.
  • 3Ponchel F, Legier J F, Soyer C, et al. Rigorous Extraction Tunability of Si-intega'ated Bao.3Sro.7TiO3 Thin Film up to 60 GHz[ J]. Appl. Phys. Lett. ,2010,96:252906.
  • 4Alldredge L M B, Chang W, Kirchoefer S W, et al. Microwave Dielectric Properties of BaTiO3 and Ba0.5Sro.sTiO3 Thin Films on (001) MgO [ J]. Appl. Phys. Lett. ,2009,95:222902.
  • 5Xiao B, Liu H R, Avrutin V, et al. Epitaxial Growth of (001)-oriented B%.sSr0.sTiO3 Thin Films on a-plane Sapphire with an MgO/ZnO Bridge Layer[ J ]. Appl. Phys. Lett. ,2009,95:212901.
  • 6Wu J, Wang J, Xiao D Q, et al. Leakage Mechanism of Cation-modified BiFeO3 Thin Film[J]. AIP Adu. ,2011, ( 1 ) :022138.
  • 7Yang H, Jain M, Suvorova N A, et al. Temperature-dependent Leakage Mechanisms of Pt/BiFeO3/SrRuO3 Thin Film Capacitors [ J ]. Appl. Phys. Lett. ,2007,91:072911.
  • 8Nagaraj B, Aggarwal S. Leakage Current Mechanisms in Lead-based Thin Film Ferroelectric Capacitors [ J ]. Phys. Rev. B, 1999,59:16022- 16026.
  • 9Pabst G W, Martin L W, Chu Y H, et al. Leakage Current Mechanisms in BiFeO3 Thin Films[ J]. Appl. Phys. Lett. ,2007,90:072902.
  • 10Akhan M, Comyn T, Bell A J. Leakage Mechanisms in Bismuth Ferrite-lead Titanate Thin Films on Pt/Si Substrates [ J ]. Appl. Phys. Lett. ,2008, 92 : 072908.

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