摘要
We investigate multiphoton ionization （MPI） of N2 exposed to femtosecond laser fields at 400nm and 80Onto experimentally. Photoelectron energy spectra are measured with a high resolution photoelectron spectrometer at laser intensities up to 10^14 W/cm^2. Prominent resonant peaks observed at 400nm can be attributed to the resonance with molecular Rydberg states corresponding to different molecular orbitals, revealing the importance of the multiple orbitals contribution in strong field molecular dynamics.
We investigate multiphoton ionization （MPI） of N2 exposed to femtosecond laser fields at 400nm and 80Onto experimentally. Photoelectron energy spectra are measured with a high resolution photoelectron spectrometer at laser intensities up to 10^14 W/cm^2. Prominent resonant peaks observed at 400nm can be attributed to the resonance with molecular Rydberg states corresponding to different molecular orbitals, revealing the importance of the multiple orbitals contribution in strong field molecular dynamics.
基金
Supported by the National Natural Science Foundation of China under Grant Nos 10925420 and 10904162, and the Natural Science Foundation of Hubei Province under Grant No 2008CDB007.
