期刊文献+

Fe^(3+)/Al^(3+)-TiO_2复合光催化剂的制备及其光催化性能研究 被引量:5

Preparation and photocatalytic activity of Fe^(3+)/Al^(3+)-TiO_2 composite photocatalyst and its the photocatalytic activity
下载PDF
导出
摘要 以钛酸四正丁酯为先驱物,采用溶胶-凝胶法制备铁铝共掺杂的TiO2(Fe3+/Al3+-TiO2)复合光催化剂,并用XRD、UV-Vis等进行表征,系统研究煅烧温度、光催化体系中的盐对Fe3+/Al3+-TiO2复合光催化剂在自然光条件下光催化降解甲基橙性能的影响。结果表明,Fe3+/Al3+-TiO2光催化降解甲基橙的性能随着煅烧温度的升高而增强,催化体系中的HCO3-和NO2-使Fe3+/Al3+-TiO2复合光催化剂的催化活性有所降低。 Fe3+ and Al 3+ co-doped TiO2(Fe^3+/Al^3+-TiO2)composite photocatalysts were prepared by the sol-gel method using Ti(OC4H9)4 as precursor and characterized by X-ray diffraction(XRD)and UV-Vis.The effect of calcination temperature and salts in photocatalytic system on the photocatalytic activity of Fe^3+/Al^3+-TiO2 were investigated by photocatalytic degradation of methyl orange irradiated by sunlight.The photocatalytic activity of Fe^3+/Al^3+-TiO2 was enhanced with increasing temperature.HCO3-and NO2-decreased its photocatalytic activity.
出处 《功能材料》 EI CAS CSCD 北大核心 2010年第11期1896-1899,共4页 Journal of Functional Materials
基金 国家自然科学基金资助项目(30672103) 江西省教育厅重点科技资助项目(DB200802094)
关键词 溶胶-凝胶法 铁铝共掺杂 二氧化钛 自然光 光催化降解 sol-gel method Fe3+and Al 3+co-doped titania nature light photocatalytic degradation
  • 相关文献

参考文献21

  • 1Sun B, Vorontsov A V, Smirniotis P G. [J]. Langmuir, 2003: 19: 3151-3256.
  • 2Bejarano-Perez N J, Suarez-Herrera M F. [J]. Ultra Sonochem, 2007, 14: 589-595.
  • 3Gratzei M, Howe R F, [J]. J Phys Chem, 1990, 94: 2566-2572.
  • 4Asahi R, Morikawa T, Ohwahi T, et al. [J]. Science, 2001, 293,. 269-271.
  • 5Tada H, Hattori A, Tokihisa Y, et al. [J]. J Phys Chem B, 2000, 104: 4585-4587.
  • 6Hu C, Tang Y, Yu J C,et al.[J]. Appl Catal B: Environ, 2003, 40(2): 131-140.
  • 7Kawahara T, Konishi Y, Tada H, et al. [J]. Langmuir, 2001, 17: 7442-7446.
  • 8Tada H, Konishi Y, Kokubu A, et al. [J]. Langmuir, 2004, 20: 3816-3819.
  • 9Cao Y, Zhang X, Yang W, et al. [J]. Chem Mater, 2000, 12: 3445-3448.
  • 10Linsebigier A L, Lu G Q, Yates T. [J]. Chem Rev, 1995, 95(3): 735-758.

同被引文献75

  • 1Wu D, Long M. Realizing visible-light-induced self- cleaning property of cotton through coating N-TiO2 film and loading AgI particles [ J ]. ACS Appl. Mater. Interfaces,2011,3:4770 - 4774.
  • 2Yang L, Luo S, Li Y, et al. High efficient photocatalyt- ic degradation of p-nitrophenol on a unique Cu20! TiO2 p-n heterojunction network catalyst[ J]. Environ. Sci. Technol. ,2010,44:7641 - 7646.
  • 3Jin Y, Zhao G, Wu M, et al. In situ induced visible- light photoeletrocatalytic activity from molecular oxy- gen on carbon aerogel-supported TiO2 [ J ]. J. Phys. Chem. C ,2011,115:9917 - 9925.
  • 4Wang H, Duan J, Cheng Q. Photocatalytically pat- terned TiO2 arrays for on-plate selective enrichment of phosphopeptides and direct MALDI MS analysis [ J ]. Anal. Chem. ,2011,83 : 1624 - 1631.
  • 5Stengl V, Popelkov6 D, V16 il P. TiO2 -graphene nano- composite as high performace photocatalysts [ J ]. J Phys Chem C ,2011,115:25209 - 25218.
  • 6Singh A P, Kumari S, Shrivastavb R, et al. Iron doped nanostructured TiO2 for photoelectrochemical genera- tion of hydrogen[ J ]. Int. J. Hydrog. Energy,2008,33 : 5363 - 5368.
  • 7Torrell M ,Cunha L,Kabir Md R,et al. Nanoscale col- or control of TiO2 lms with embedded Au nanoparti- cles [ J ]. Mater. Lett. ,2010,64:2624 - 2626.
  • 8Yoon J, Shim E, Bae S, et al. Application of immobi- lized nanotubular TiO2 electrode for photocatalytic hy-drogen evolution:Reduction of hexavalent chromium ( Cr (VI) ) in water [ J ]. J. Hazard. Mater. , 2009, 161:1069 - 1074.
  • 9Sohn Y S, Smith Y R, Subramanian V R, et al. Elec- trochemically assisted photocatalytic degradation of methyl orange using anodized titanium dioxide nano- tubes [ J ]. Appl. Catal. B ,2008,84 : 372 - 378.
  • 10Kar A, Smith Y R,Subramanian V R. Improved photo- catalytic degradation of textile dye using titanium di- oxide nanotubes formed over titanium wires I J 1- Envi- ron. Sei. Technol. ,2009,43:3260 - 3265.

引证文献5

二级引证文献14

相关作者

内容加载中请稍等...

相关机构

内容加载中请稍等...

相关主题

内容加载中请稍等...

浏览历史

内容加载中请稍等...
;
使用帮助 返回顶部