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半导体纳米颗粒电子的超快弛豫过程

Electron Ultrafast Relaxation Process in Semiconductor Nanoparticles
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摘要 为了研究在飞秒激光作用下半导体纳米颗粒的超快动力学过程,建立了一个带表面态的三能级结构的载流子弛豫简化模型,得出各能级的电子速率方程.利用数值模拟方法模拟出各能级电子密度和差分吸收率随时间的变化情况,得知由于吸收截面的变化,差分吸收谱会有一个超快的变化过程.并将模拟结果与FanxinWu等人的实验结果相比较,其曲线特征基本一致.说明该模型有一定的合理性. To study the dynamic process excited by femtsecond laser,a carrier model with three energy level and trap is constructed,with which the electron rate equation is obtained.The numerical simulation is used to calculate the electron number change of each energy level and the differentiated absorbtion rate as the time goes by.With the change of the electron's absorption cross-section,differentiated absorbtion rate will have a ultrafast change process.Compared with the experimental result of Fanxin Wu,the differentiated absorbtion rate curves are basically the same,which shows the model have some rationality.
出处 《光子学报》 EI CAS CSCD 北大核心 2010年第10期1738-1741,共4页 Acta Photonica Sinica
基金 国家重点基础研究发展计划(2007CB307002)资助
关键词 半导体纳米颗粒 载流子弛豫 速率方程 数值模拟 Semiconductor nanoparticle Carrier relaxation Rate equation Numerical simulation
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参考文献16

  • 1ELSAESSER T,WOERNER M.Femtosecond infrared spectroscopy of semiconductors and semiconductor nanostructures[J].Phy Rep,1999,321(6):253-305.
  • 2李霞,姚保利,侯洵.以衍射理论为基础考虑双光子吸收的Z-扫描理论[J].光子学报,2005,34(7):1010-1014. 被引量:6
  • 3姚保利,任立勇,侯洵.基于衍射模型的Z扫描理论[J].光学学报,2002,22(1):19-23. 被引量:15
  • 4胡建莉,丁迎春.基于衍射理论的大非线性相移Z扫描研究[J].光子学报,2008,37(11):2163-2166. 被引量:3
  • 5BARTELS A, HUDERT F, JANKE C, et al. Femtosecond time-resolved optical pump-probe spectroscopy at kilohertz-scan-rates over nanosecond-time-delays without mechanical delay line[J]. Applied Physics Letters, 2006, 88(041117):1-3.
  • 6BOOK L D,ARNETT D C,HU H,et al.Ultrafast pump-probe studies of excited-state charge-transfer dynamics in blue copper proteins[J]. J Phys Chem A,1998,102(23):4350-4359.
  • 7ZHANG J Z ,O′NEIL R H ,ROBERTI T W .Femtosecond studies of photoinduced electron dynamics at the liquid-solid interface of aqueous CdS colloids[J].J Phys Chem,1994,98(14):3859-3864.
  • 8ROBERTI T W, CHEREPY N J, ZHANG J Z. Nature of the power-dependent ultrafast relaxation process of photoexcited charge carriers in II-VI cemiconductor quantum dots:Effects of particle size,surface and electronic structurep[J].J Chem Phys,1998,108(5):2143-2151.
  • 9ZHANG J Z,O′NEIL R H,ROBERTI T W,et al.Femtosecond studies of trapped electrons at the liquid-solid interface of aqueous CdS colloids[J].Chem Phys lett,1994,218(5-6):479-484.
  • 10WU Fan-xin,YU Jung-ho,JOO Jin.Ultrafast electronic dynamics of monodisperse PbS and CdS nanoparticles nanorods Effects of size on nonlinear relaxation[J].Opt Mater,2007,29(7):858-866.

二级参考文献26

  • 1李霞,姚保利,侯洵.以衍射理论为基础考虑双光子吸收的Z-扫描理论[J].光子学报,2005,34(7):1010-1014. 被引量:6
  • 2SHEIK-BAHAE M, SAID A A, WEI T, et al. Sensitive measurement of optical nonlinearities using a single beam[J]. IEEE Jounal of Quantum Electronics ,1990,26(4) :760-769.
  • 3YAO Bao-li, REN Li-yong, HOU Xun. Z-scan theory on a diffraction model[J]. JOSA B,2003,20(6) : 1290-1294.
  • 4[1]COMIN A,GIANNETTI C,SAMOGGIA G at al.Elastic and Magnetic Dynamics of Nanomagnet-Ordered Arrays Impulsively Excited by Subpicosecond Laser Pulses[J].Physical Review-Letters,2006,97(217201):1-4.
  • 5[2]LIU Hong-ping,YIN Shu-hui,ZHANG Jian-yang,et al.Femtosecond resonance-enhanced multiphoton-ionization photoelccuron spectrum of ammonia[J].Physical Review A,2006,74(053418):1-5.
  • 6[3]BARTELS A,HUDERT F,JANKE C,et al.Femtosecond time-resolved optical pump-probe spectroscopy at kilohertz-Sean-rates over nanosecond-time-delays without mechanical delay line[J].Appfied Physics Letters,2006,88(041117):1-3.
  • 7[4]KUTHIRUMMAL N,RUDAKOV F M,EVANS C L,et al.Spectroscopy and femtosecond dynamics of the ring opening reaction of 1,3-cyclohexadiene[J].The Journal of Chemical Physics,2006,125(133307):1-8.
  • 8[5]RAO S V,RAO D N,AKKARA J A,et al.Dispersion studies of non-linear absorption in C60 using Z-scan[J].Chemical Physics Letters,1998,297:491-498.
  • 9[6]SRINlVAS N K M N,RAO S V,RAO D N.Saturable and rcverse saturable absorption of Rhodamine B in methanol and water[J].J Opt Sec Am B,2003,20(12):2470-2479.
  • 10[7]WANG J,BAHAE M S,SAID A A et al.Time-resolved Z-scan measurements of optical nonlinearities[J].J Opt Soc Am B,1994,11(6]:1009-1017.

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