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荧光染料掺杂DNA-CTMA薄膜的放大自发辐射特性 被引量:6

Amplified Spontaneous Emission of Fluorescent Dye-Doped DNA-CTMA Thin Films
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摘要 采用旋涂法制备了若丹明6G(Rh6G)和若丹明B(RhB)两种染料掺杂的DNA-CTMA复合薄膜,并通过对薄膜的表面形貌、紫外/可见/红外吸收光谱、荧光光谱特性的测量,表征了薄膜的成膜质量及光谱特性。通过Nd∶YAG脉冲激光器的倍频光激发,研究了不同比例荧光染料掺杂DNA-CTMA薄膜的放大自发辐射(ASE)现象并做了理论解释。实验结果表明,在波长为532 nm的脉冲激光抽运下,Rh6G/RhB/DNA-CTMA薄膜的发射谱出现了明显的窄化现象,而且比单一染料掺杂DNA-CTMA薄膜的发射谱呈现出较大的光谱调谐范围,是一种较好的有机聚合物激光材料体系。 The fluorescent dye Rhodamine-6G (Rh6G) and Rhodamine-B (RhB) doped DNA-CTMA thin films are prepared by spin-coating technology. The quality and optical spectra properties of Rh6G/RhB/DNA-CTMA thin films are characterized by the measurements of surface morphology, UV/vis/infrared absorption spectra and fluorescence spectra. The amplified spontaneous emission (ASE) of dye-doped DNA-CTMA thin films with different dye contents was researched experimentally by pumping of Nd: YAG pulse laser at wavelength of 532 nm, and is explained theoretically. The experimental results show that the narrowing phenomenon of emission spectra of Rh6G/RhB/DNA- CTMA thin films is very clear and strong. Compared with single dye doped DNA-CTMA thin films, the co-doped Rh6G/RhB/DNA-CTMA thin film is a potential candidate as an organic polymer laser material because it exhibits more wider tuning range of the ASE spectrum.
出处 《中国激光》 EI CAS CSCD 北大核心 2011年第5期175-180,共6页 Chinese Journal of Lasers
基金 国家自然科学基金(60977048) 浙江省钱江人才计划(2009R10064) 宁波市国际科技合作计划(2010D10018)资助课题
关键词 薄膜 若丹明6G 若丹明B DNA—CTMA 放大自发辐射 thin films Rhodamine 6G Rhodamine B DNA-CTMA amplified spontaneous emission
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  • 1Lili Wang, Jonichi Yoshida, Naoya Ogata. Self-assembled supramolecular films derived from marine deoxyribonucleic acid (DNA)-cationic surfactant complexes:large-scale preparation and optical and thermal properties[J]. Chem. Mater., 2001, 13(4): 1273-1281.
  • 2P. Yaney, E. Heckman, D. Diggs et al.. Development of chemical sensors using polymer optical waveguides fabricated with DNA[C]. SPIE, 2005, 5724: 224-233.
  • 3J. A. Hagen, W. Li, A. J. Steckla et al.. Enhanced emission efficiency in organic light-emitting diodes using deoxyribonucleic acid complex as an electron blocking layer[J]. Appl. Phys. Lett., 2006, 88(17): 171109.
  • 4F. Puntoriero, S. Campagna, M. L. Di Pietro et al.. Luminescence of a Pt(II) complex in the presence of DNA. Dependence of luminescence changes on the interaction binding mode[J]. Photochem. Photobiol. Sci., 2007, 6(4): 357-360.
  • 5Philipp Stadler, Kerstin Oppelt, Thokchom Birendra Singh et al.. Organic field-effect transistors and memory elements using deoxyribonucleic acid (DNA) gate dielectric[J]. Organic Electronics, 2007, 8(6): 648-654.
  • 6谢旭东,胡丽丽,黄国松,姜中宏.高分子基体的固体染料激光器的制备和研究[J].中国激光,2000,27(4):307-311. 被引量:5
  • 7L. Wang, K. Ishihara, H. Izumi et al.. Strongly luminescent rare-earth ion-doped DNA-CTMA complex film and fiber materials[C]. SPIE, 2002, 4905: 143-153.
  • 8Z. Yu, W. Li, J. A. Hagen et al.. Photoluminescence and lasing from deoxyribonucleic acid (DNA) thin films doped with sulforhodamine[J]. Appl. Opt., 2007, 46(9): 1507-1513.
  • 9Y. Kawabe, L. Wang, S. Horinouchi et al.. Amplified spontaneous emission from fluorescent-dye-doped DNA-surfactant complex films[J]. Advan. Materials, 2000, 12(17): 1281-1283.
  • 10Y. Kawabe, L. Wang, T. Nakamura et al.. Thin-film lasers based on dye-deoxyribonucleic acid-lipid complexs[J]. Appl. Phys. Lett., 2002, 81(8): 1372-1374.

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  • 1Steckl A J, Spaeth H, Singh K, et al. Chirality of sulforhodamine dye molecules incorporated in DNA thin films[J]. Appl Phys Lett, 2008 93 : 193903.
  • 2Kawabe Y, Wang L, Horinouchi S, et al. Amplified spontaneous emission from fluorescent-dye-doped DNA-surfactant complex films[J]. Adv Mater, 2000, 12(17) : 1281-1283.
  • 3Kawabe Y, Wang L, Nakamura T, et al. Thin films lasers based on dye deoxyribonucleic acid-lipid complexes[J]. Appl Phys Lett, 2002, 81(8):1372- 1374.
  • 4Yu Z, Li W, Hagen J A, et al. Photoluminescence and lasing from deoxyribonculeicacid (DNA) thin films doped with sulforhodamine[J]. ApplOpt, 2007, 46(9) :1507-1513.
  • 5Mysliwiec J, Sznitko L, Bartkiewicz S, et al. Amplified spontaneous emission in the spiropyran-biopolymer based system[J]. Appl PhysLett, 2009, 94:241106.
  • 6Mysliwiec J, Sznitko L, Miniewicz A. et al. Study of'the amplified spontaneous emission in a dye-doped biopolymer-based material[J]. J Phys D :Appl Phys, 2009, 42 : 085101.
  • 7Mysliwiec J, Sznitko L, Sobolewska A. et al. Lasing effect in a hybrid dye-doped biopolymer and photochromic polymer system[J]. Appl Phys Lett, 2010, 96:141106.
  • 8Tsang K C, Wong C Y, Pun E Y B. Optical amplification in Eu3+-doped DNA based biopolymer[J]. Phot Tech Lett, 2011,23(16) :1106- 1108.
  • 9Heliotis G, Choulis S A, Itskos G, et al. Low threshold lasers based on a high-mobility semiconducting polymer[J]. Appl Phys Lett, 2006, 88 : 081104.
  • 10Ribierre J C, Tsiminis G, Richardson S, et al. Amplified spontaneous emission and lasing properties of bisfluorenecored dendrimers[J]. Appl Phys Lett, 2.007, 91:081108.

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