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Characteristics of sulfate in atmosphere over Xiamen waters and its fluxes to waters

Characteristics of sulfate in atmosphere over Xiamen waters and its fluxes to waters
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摘要 One hundred and seven marine aerosol samples were collected during December 1988 to March 1990, and 3 dry deposition samples, 16 rain samples and 2 Cascade Impacter samples were collected from March to May 1990 at the southeast coast of the Xiamen Island. All the samples were analyzed for SO42-, NO3-, Cl-, Na+ , NH4+, using ion chromatography.The results indicate that the concentration of sulfate in marine aerosols over the Xiamen waters appears to be of seasonal variation, in an order of winter > spring > autumn > summer. The mean sulfate concentration lor the total marine aerosol samples over the Xiamen waters is 9. 37 μg/m3, respectively 0. 89 and 8. 48 μg/m3 for the seasalt and non-sea-salt sulfate. The distribution of sulfate shows a bimodal form with a peak in the coarse particle range which is derived from the sea-salt sulfate, and a peak in the fine particle range which is derived from the non-sea-salt sulfate. The total deposition of sulfate to the Xiamen waters is estimated to be 4. 68g/m2 · a, with dry and wet depositions being approximately 2.19 and 2. 49g/m2 · a respectively. One hundred and seven marine aerosol samples were collected during December 1988 to March 1990, and 3 dry deposition samples, 16 rain samples and 2 Cascade Impacter samples were collected from March to May 1990 at the southeast coast of the Xiamen Island. All the samples were analyzed for SO42-, NO3-, Cl-, Na+ , NH4+, using ion chromatography.The results indicate that the concentration of sulfate in marine aerosols over the Xiamen waters appears to be of seasonal variation, in an order of winter > spring > autumn > summer. The mean sulfate concentration lor the total marine aerosol samples over the Xiamen waters is 9. 37 μg/m3, respectively 0. 89 and 8. 48 μg/m3 for the seasalt and non-sea-salt sulfate. The distribution of sulfate shows a bimodal form with a peak in the coarse particle range which is derived from the sea-salt sulfate, and a peak in the fine particle range which is derived from the non-sea-salt sulfate. The total deposition of sulfate to the Xiamen waters is estimated to be 4. 68g/m2 · a, with dry and wet depositions being approximately 2.19 and 2. 49g/m2 · a respectively.
出处 《Acta Oceanologica Sinica》 SCIE CAS CSCD 1993年第4期585-595,共11页 海洋学报(英文版)
关键词 SULFATE marine aerosol Xiamen waters Sulfate, marine aerosol, Xiamen waters
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