乙烯分子在激光场中的多光子电离及高次谐波的产生

High-order harmonic generation and multi-photon ionization of ethylene in laser fields

本文运用含时密度泛函理论和局域密度近似方法,分别研究了乙烯分子在单色激光场、双色激光场中电离和高次谐波的产生。计算结果表明,在单色激光场中,乙烯分子的高次谐波谱呈现出明显的平台区和奇次谐波加强的特征:在双色激光场中,乙烯分子的电离增强而出现高电荷态几率,并伴有偶次谐波的出现。

Applying the time dependent local density approximation（TDLDA）,the high-order harmonic generation（HHG）spectra and the ionization probabilities of ethylene subject to the one-colour and two-colour laser field are explored.It is found that HHG spectra of ethylent exhibits the plateau obviously from the fifth order to the ninth order harmonic and the odd harmonics are strengthed in the one-colour laser field.Furthermore,the ionization of ethylene is enhanced in the two-colour laser field resulting the appearance of the high charge state and the even harmonics.