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Transport simulation of sorptive contaminants considering sediment-associated processes

Transport simulation of sorptive contaminants considering sediment-associated processes
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摘要 Sediment-associated processes, such as sediment erosion, deposition, and pore water diffusion/advection affect sorptive contaminant transport. By considering these processes, we developed an equation to simulate contaminant transport. Erosion and deposition processes are considered as erosion and deposition fluxes of sediment, and adsorption-desorption processes of contaminants by sediment are simulated using the Langmuir Equation. Pore water diffusion is calculated based on the contaminant concentration gradient across the sediment-water interface. Pore water advection is estimated using pore water contained in the sediments of erosion flux. The equation is validated to simulate total phosphorus concentrations in Guanhe estuary in the northern Jiangsu, China. The simulated total phosphorus concentrations show better agreement with field observations compared to estimations that do consider sediment-associated processes. Sediment-associated processes, such as sediment erosion, deposition, and pore water diffusion/advection affect sorptive contaminant transport. By considering these processes, we developed an equation to simulate contaminant transport. Erosion and deposition processes are considered as erosion and deposition fluxes of sediment, and adsorption-desorption processes of contaminants by sediment are simulated using the Langmuir Equation. Pore water diffusion is calculated based on the contaminant concentration gradient across the sediment-water interface. Pore water advection is estimated using pore water contained in the sediments of erosion flux. The equation is validated to simulate total phosphorus concentrations in Guanhe estuary in the northern Jiangsu, China. The simulated total phosphorus concentrations show better agreement with field observations compared to estimations that do consider sediment-associated processes.
出处 《Chinese Journal of Oceanology and Limnology》 SCIE CAS CSCD 2012年第4期668-674,共7页 中国海洋湖沼学报(英文版)
基金 Supported by the Specialized Research Fund for the Doctoral Program of Higher Education of China(No.200802940014)
关键词 sorptive contaminant SEDIMENT transport equation Guanhe estuary 污染物运移 交通模拟 吸附解吸 泥沙 Langmuir方程 侵蚀通量 运移方程 沉积过程
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