摘要
We propose a catalysis-select migration driven evolution model of two-species（A-and B-species） aggregates,where one unit of species A migrates to species B under the catalysts of species C,while under the catalysts of species D the reaction will become one unit of species B migrating to species A.Meanwhile the catalyst aggregates of species C perform self-coagulation,as do the species D aggregates.We study this catalysis-select migration driven kinetic aggregation phenomena using the generalized Smoluchowski rate equation approach with C species catalysis-select migration rate kernel K（k;i,j） = Kkij and D species catalysis-select migration rate kernel J（k;i,j） = Jkij.The kinetic evolution behaviour is found to be dominated by the competition between the catalysis-select immigration and emigration,in which the competition is between JD0 and KC0（D0 and C0 are the initial numbers of the monomers of species D and C,respectively）.When JD0 KC0 〉 0,the aggregate size distribution of species A satisfies the conventional scaling form and that of species B satisfies a modified scaling form.And in the case of JD0 KC0 〈 0,species A and B exchange their aggregate size distributions as in the above JD0 KC0 〉 0 case.
We propose a catalysis-select migration driven evolution model of two-species（A-and B-species） aggregates,where one unit of species A migrates to species B under the catalysts of species C,while under the catalysts of species D the reaction will become one unit of species B migrating to species A.Meanwhile the catalyst aggregates of species C perform self-coagulation,as do the species D aggregates.We study this catalysis-select migration driven kinetic aggregation phenomena using the generalized Smoluchowski rate equation approach with C species catalysis-select migration rate kernel K（k;i,j） = Kkij and D species catalysis-select migration rate kernel J（k;i,j） = Jkij.The kinetic evolution behaviour is found to be dominated by the competition between the catalysis-select immigration and emigration,in which the competition is between JD0 and KC0（D0 and C0 are the initial numbers of the monomers of species D and C,respectively）.When JD0 KC0 〉 0,the aggregate size distribution of species A satisfies the conventional scaling form and that of species B satisfies a modified scaling form.And in the case of JD0 KC0 〈 0,species A and B exchange their aggregate size distributions as in the above JD0 KC0 〉 0 case.
基金
Project supported by the National Natural Science Foundation of China (Grant Nos. 10875086 and 10775104)
