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Optical and thermoluminescence properties of Lu_2Si_2O_7:Pr single crystal

Optical and thermoluminescence properties of Lu_2Si_2O_7:Pr single crystal
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摘要 Single crystal of Lu2Si2OT:Pr was grown by Czochralski method. Transmittance, photoluminescence excitation (PLE) and photo- luminescence (PL) spectra, X-ray excited luminescence (XEL) and fluorescence decay time spectra of the sample were measured and dis- cussed to investigate its optical characteristics. The crystal structure of the as grown Lu2Si207:Pr was confirmed to be C2/m. There was a broad absorption peaking at 245 um in the region from 200-260 urn. The PL spectntm was dominated by fast 3py^3Hj band peaking at 524 nm. The XEL spectrum was dominated by the fast 5d14t^---~41e emission peaking at 265 nm. The 2D (temperature-intensity) and 3D (tem- perature-wavelength-intensity) thermally stimulated luminescence (TSL) spectra were measured. The Pr3+ ion was found to be the recombina- tion center during the TSL process. Three obvious traps were detected in LPS:Pr single crystal with energy depth at 1.06, 0.78 and 0.67 eV. Single crystal of Lu2Si2OT:Pr was grown by Czochralski method. Transmittance, photoluminescence excitation (PLE) and photo- luminescence (PL) spectra, X-ray excited luminescence (XEL) and fluorescence decay time spectra of the sample were measured and dis- cussed to investigate its optical characteristics. The crystal structure of the as grown Lu2Si207:Pr was confirmed to be C2/m. There was a broad absorption peaking at 245 um in the region from 200-260 urn. The PL spectntm was dominated by fast 3py^3Hj band peaking at 524 nm. The XEL spectrum was dominated by the fast 5d14t^---~41e emission peaking at 265 nm. The 2D (temperature-intensity) and 3D (tem- perature-wavelength-intensity) thermally stimulated luminescence (TSL) spectra were measured. The Pr3+ ion was found to be the recombina- tion center during the TSL process. Three obvious traps were detected in LPS:Pr single crystal with energy depth at 1.06, 0.78 and 0.67 eV.
出处 《Journal of Rare Earths》 SCIE EI CAS CSCD 2012年第8期775-779,共5页 稀土学报(英文版)
基金 Project supported by National Natural Science Foundation of China(50902145,51171239) the Natural Science Foundation of Shanghai(09ZR1435800) the Knowledge Innovation Program of the Chinese Academy of Sciences(SCX200701)
关键词 Pr3+ doped lutetium pyrosilicate single crystal scintillation optical properties thermally stimulated luminescence rare earths Pr3+ doped lutetium pyrosilicate single crystal scintillation optical properties thermally stimulated luminescence rare earths
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