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针-板式介质阻挡放电降解土壤中对硝基苯酚研究

Degradation of p-Nitrophenol in Soil Using Needle-Plate Dielectric Barrier Discharge
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摘要 采用针-板式介质阻挡放电(DBD)产生低温等离子体降解土壤中对硝基苯酚(PNP),考察了放电电压、载气气量、土壤含水率以及土壤pH值对土壤中PNP降解效果的影响。结果表明:针-板式DBD对土壤中PNP有良好的降解效果。在PNP初始浓度400mg/kg,放电电压18 kV条件下,放电处理60 min,PNP降解率达到87.3%。增加放电电压和含水率均能提高降解率。不通入载气,也有较好的降解效果。碱性条件有利于PNP降解。 Non-thermal plasma produced by needle-plate dielectric barrier discharge(DBD) was developed to investigate the degradation of p-nitrophenol(PNP) in soil.Effects of discharge voltage,air flow rate,soil moisture content and soil pH on PNP degradation were evaluated.Experimental results showed that the needle-plate DBD system has a favorable removal efficiency for PNP.About 87.3% of PNP could be removed after 60min DBD decomposition with initial concentration 400 mg/kg and discharge voltage 18 kV.Increasing the discharge voltage and soil moisture content could both improve the degradation efficiency and a better PNP degradation was obtained without air flow rate.Alkaline soil was favorable for PNP removal.
出处 《环境科学与技术》 CAS CSCD 北大核心 2012年第10期50-52,57,共4页 Environmental Science & Technology
基金 国家自然科学基金项目(40901150)
关键词 介质阻挡放电(DBD) 土壤 对硝基苯酚 降解 dielectric barrier discharge(DBD) soil p-nitrophenol(PNP) degradation
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参考文献11

  • 1Rogers KR, van Emon J M. Immunoassay for p-nitrophenol in Urine[R]. 1993 ,EPA Report No. EPAI6001A-931074, USA.
  • 2Uberoi V, Bhattacharya S K. Toxicity and degradability of nitrophenols in aerobic systems[J]. Water Environment Re- search, 1997, 69(2) : 146-156.
  • 3Feng J W, Zheng Z, Sun Y B, et al. Degradation of diuron in aqueous solution by dielectric barrier discharge[J]. Journal of Hazardous Materials, 154:1081-1089.
  • 4Magureanu M, Piroi D, Mandache N B, et al. Degradation of pharmaceutical compound pentoxifylline in water by non-thermal plasma treatment[J]. Water Resource, 2010 (44): 3445-3453.
  • 5Liang Wen-jun, Li Jian, Li Jie, et al. Abatement of toluene from gas streams via ferro-electric packed bed dielectric barrier discharge plasma[J]. Journal of Hazardous Materials, 2009( 170 ):633--638.
  • 6Lukes P, Clupek M, Babicky V, et al. Generation of ozone by pulsed corona discharge over water surface in hybrid gas-liquid electrical discharge reactor[J]. Journal of Physics D: Applied Physics, 2005(38):409-416.
  • 7Wang J X, Chen S, Quan X, et al. Enhanced photodegrada- tion of PNP on soil surface under UV irradiation with TiO2 [J]. Soil Sediment Contam,2007(16):413--421.
  • 8Wang T C, Lu N, Li J, et al. Evaluation of the potential of pentachlorophenol degradation in soil by pulsed corona dis-charge plasma from soil characteristics[J]. Environ Sci- ence & Technology, 2010(44):3105-3110.
  • 9Wang T C, Lu N, Li J, et al. Enhanced Degradation of p- nitrophenol in soil in a pulsed discharge[J]. Journal of Hazardous Materials, 2011(11):276-280.
  • 10Feng J W, Zheng Z, Luan J F, et al. Gas-liquid hybrid discharge-induced degradation of diuron in aqueous solution [J]. Journal of Hazardous Materials, 2009,164(2-3): 838-846.

二级参考文献12

  • 1辛力锋,朱天宇,卞新高,钱雪松,陈静,赵达.冷却条件对高频臭氧发生器产量的影响分析[J].河海大学常州分校学报,2004,18(4):19-21. 被引量:3
  • 2MOK Y S, KIM K T. Demonstration of flue gas cleaning by positive pulsed corona discharge process [J]. Conference Record of the 1999 IEEE, 1999, 1(3-7):20 - 27.
  • 3NAKAJIMA N, HORINOCHI T. Ozone generator for small capacity ozone generation by using a ceramic transformer[J]. Ozone Science and Engineering, 2002, 24 (3):215-219.
  • 4ELIASSON B, KOGELSCHATZ U. Modeling and applications of silent discharge plasmas[J]. IEEE Transactions on Plasma Science, 1991,19 ( 2 ) : 309 - 323.
  • 5GUTIERREZ-TAPIA C. Dynamics of ozone generation in a silent oxygen discharge [J]. IEEE Transactions on Plasma Science, 1998, 26(4) :1357 - 1362.
  • 6KUANG Guang-li, HU Yue-xiu, SHAN Jia-fang, et al. A lower-hybrid current drive system on the superconductive Tokamak HT-7 [J]. Fusion Technology, 1999, 36(2):212-218.
  • 7EBIHARA K, TAKAYAMA M, STRYCZEWSKA H, et al. Ozone generation by dielectric barrier discharge for soil sterilization[J]. Thin Solid Films, 2006, 506-507: 396 -399.
  • 8ULRICH K. Dielectric barrier discharges: their history, discharge physics, and industrial applications[J].Plasma Chemistry and Plasma Processing, 2003, 23 (1) 1 -46.
  • 9YOUL M S, TATSUYA S. Optimum conditions for ozone formation in a micro dielectric barrier discharge[J]. Surface & Coatings Technology, 2005, 197 : 148 - 153.
  • 10张波,岳朝松,储金宇,陈万金.臭氧发生器运行参数的正交试验研究[J].高电压技术,2002,28(10):43-44. 被引量:2

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