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Emission inventory evaluation using observations of regional atmospheric background stations of China 被引量:7

Emission inventory evaluation using observations of regional atmospheric background stations of China
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摘要 Any accurate simulation of regional air quality by numerical models entails accurate and up-to-date emissions data for that region.The INTEX-B2006 (I06),one of the newest emission inventories recently popularly used in China and East Asia,has been assessed using the Community Multiscale Air Quality model and observations from regional atmospheric background stations of China.Comparisons of the model results with the observations for the species SO2,NO 2,O 3 and CO from the three regional atmospheric background stations of Shangdianzi,Longfengshan and Linan show that the model can basically capture the temporal characteristics of observations such as the monthly,seasonal and diurnal variance trends.Compared to the other three species,the simulated CO values were grossly underestimated by about two-third or one-half of the observed values,related to the uncertainty in CO emissions.Compared to the other two stations,Shangdianzi had poorer simulations,especially for SO2 and CO,which partly resulted from the site location close to local emission sources from the Beijing area;and the regional inventory used was not capable of capturing the influencing factors of strong regional sources on stations.Generally,the fact that summer gave poor simulation,especially for SO2 and O 3,might partly relate to poor simulations of meteorological fields such as temperature and wind. Any accurate simulation of regional air quality by numerical models entails accurate and up-to-date emissions data for that region.The INTEX-B2006 (I06),one of the newest emission inventories recently popularly used in China and East Asia,has been assessed using the Community Multiscale Air Quality model and observations from regional atmospheric background stations of China.Comparisons of the model results with the observations for the species SO2,NO 2,O 3 and CO from the three regional atmospheric background stations of Shangdianzi,Longfengshan and Linan show that the model can basically capture the temporal characteristics of observations such as the monthly,seasonal and diurnal variance trends.Compared to the other three species,the simulated CO values were grossly underestimated by about two-third or one-half of the observed values,related to the uncertainty in CO emissions.Compared to the other two stations,Shangdianzi had poorer simulations,especially for SO2 and CO,which partly resulted from the site location close to local emission sources from the Beijing area;and the regional inventory used was not capable of capturing the influencing factors of strong regional sources on stations.Generally,the fact that summer gave poor simulation,especially for SO2 and O 3,might partly relate to poor simulations of meteorological fields such as temperature and wind.
出处 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2013年第3期537-546,共10页 环境科学学报(英文版)
基金 supported by the Chinese Ministry of Science and Technology(No.2011CB403404) the CAMS Basic Research Funds-regular(No.2010Y005) the Specific Team Fund of CAMS(No.2010Z002) the National Natural Science Foundation of China(No.40875086)
关键词 evaluation CMAQ model INTEX-B2006 inventory regional atmospheric background stations evaluation CMAQ model INTEX-B2006 inventory regional atmospheric background stations
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