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Anti-flooding of polymer electrolyte membrane fuel cell with in-plate adverse-flow flow-field

Anti-flooding of polymer electrolyte membrane fuel cell with in-plate adverse-flow flow-field
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摘要 The stoichiometric ratios and related regimes, which can promote anti-flooding of polymer electrolyte membrane fuel cell (PEMFC) with in-plate adverse-flow flow-field (IPAF), were investigated. Two flow combinations, which are the simple and complex adverse-flow between plates (ABP) that can be realized by IPAF, were employed. Constant stoichiometric ratios examination indicates that the complex ABP could improve anti-flooding of PEMFC better in the medium (greater than 200 mA/cm2 and less than 1 000 mA/cm2) and high (greater than 1 000 mA/cm2) current densities than the simple ABP. More stoichiometric ratios were introduced to find the cathode critical stoichiometry. Under the condition of cathode critical stoichiometry, the maximal local relative humidity of both electrodes of complex ABP is equal to 100% and below while the anti-flooding of the cathode of simple ABP is not satisfactory in the medium and high current densities. Further study shows that the mechanism of fuel cell, which is the imerdependence between the electrodes effect, can make significant contribution to anti-flooding. The stoichiometric ratios and related regimes, which can promote anti-flooding of polymer electrolyte membrane fuel cell (PEMFC) with in-plate adverse-flow flow-field (IPAF), were investigated. Two flow combinations, which are the simple and complex adverse-flow between plates (ABP) that can be realized by IPAF, were employed. Constant stoichiometric ratios examination indicates that the complex ABP could improve anti-flooding of PEMFC better in the medium (greater than 200 mA/cm2 and less than 1 000 mA/cm2 ) and high (greater than 1 000 mA/cm2 ) current densities than the simple ABP. More stoichiometric ratios were introduced to find the cathode critical stoichiometry. Under the condition of cathode critical stoichiometry, the maximal local relative humidity of both electrodes of complex ABP is equal to 100% and below while the anti-flooding of the cathode of simple ABP is not satisfactory in the medium and high current densities. Further study shows that the mechanism of fuel cell, which is the interdependence between the electrodes effect, can make significant contribution to anti-flooding.
出处 《Journal of Central South University》 SCIE EI CAS 2013年第4期1001-1009,共9页 中南大学学报(英文版)
基金 Project(20976095) supported by the National Natural Science Foundation of China Project(2012CB215500) supported by the National Basic Research Program of China Project(20090002110074) supported by the Specialized Research Fund for the Doctoral Program of Higher Education, China Projects(2012AA1106012, 2012AA053402) supported by the National Hi-tech Research and Development Program of China
关键词 proton exchange membrane fuel cell in-plate adverse-flow flow-field stoichiometry anti-flooding 聚合物电解质膜燃料电池 电池板 流场 质子交换膜燃料电池 化学计量比 电流密度 PEMFC ABP
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参考文献17

  • 1LIU Zhi-xiang, YANG Li-zhai, MAO Zong-qiang, ZHUGE Wei-lin, WANG Li-sheng. Behavior of PEMFC in starvation [J]. Journal of Power Sources, 2006, 157(1): 166-176.
  • 2LIANG Dong, Shen Qiang, HOU Ming, SHAO Zhi-gang, YI Bao-lian. Study of the cell reversal process of large area proton exchange membrane fuel cells under fuel starvation [J]. Journal of Power Sources, 2009, 194(2): 847-853.
  • 3GERARD M, POIROT-CROUVEZIER J P, HISSEL D, PERA M C Oxygen starvation analysis during air feeding faults in PEMFC [J] International Journal of Hydrogen Energy, 2010, 35(22) 12295-12307.
  • 4O'ROURKE A, RAMANI M, ARCAK M. In situ detection of anode flooding of a PEM fuel cell [J]. International Journal of Hydrogen Energy, 2009, 34: 6765-6770.
  • 5LIU Xuan, GUO Hang, YE Fang, MA Chong-fang. Water flooding and pressure drop characteristics in flow channels of proton exchange membrane fuel cells [J]. Electrochimica Acta, 2007, 52(11) :3607-3614.
  • 6SU Ay, WENG Fang-bor, HSU Chun-ying, CHEN Yen-ming. Studies on flooding in PEM fuel cell cathode channels [J]. International Journal of Hydrogen Energy, 2009, 34(16): 6765-6770.
  • 7O'ROURKE J, RAMANI M, ARCAK M. In situ detection of anode flooding of a PEM fuel cell [J]. International Journal of Hydrogen Energy, 2006, 31(8): 1031-1039.
  • 8KIM Sung-il, BAIK Kyung-don, KIM Beom-jun, LEE Nam-woo, KIM Min-soo. Experimental study on mitigating the cathode flooding at low temperature by adding hydrogen to the cathode reactant gas in PEM fuel cell [J]. International Journal of Hydrogen Energy, In press.
  • 9YOUSFI-STEINER N, MOCOTEGUY P, CANDUSSO D, HISSEL D, HERNANDEZ A, ASLANIDES A. A review on PEM voltage degradation associated with water management: Impacts, influent factors and characterization [J]. Journal of Power Sources, 2008,183(1):260-274.
  • 10LI Hui, TANG Yang-hua, WANG Zhen-wei, SHI Zheng, WU Shao-hong, SONG Da-tong, ZHANG Jian-lu, FATIH K, ZHANG Jiu-jun, WANG Hai-jiang, LIU Zhong-sheng, ABOUATALLAH R, MAZZA A. A review of water flooding issues in the proton exchange membrane fuel cell [J]. Journal of Power Sources, 2008, 178(1): 103-117.

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