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Radionuclides measurements and mineralogical studies on beach sands, East Rosetta Estuary, Egypt

Radionuclides measurements and mineralogical studies on beach sands, East Rosetta Estuary, Egypt
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摘要 Radiometric measurements were carried out for the beach sands from East Rosetta estuary to determine the activity concentrations of 238 U, 226 Ra, 232 Th, and 40 K, using a Hyper Pure Germanium spectrometer, to estimate the dose rates and radiation hazard indices. The average specific activities are 778.20 Bq/kg for 238 U; 646.89 Bq/kg for 226 Ra; 621.92 and 627.85 Bq/kg for the 222 Rn daughters 214 Pb and 214 Bi respectively. The average specific activity of 232 Th is 1510.25 Bq/kg, while the calculated specific activity for 40 K has an average of 8.41 Bq/kg. The average specific activity of 235 U is 38.61 Bq/kg. The average absorbed dose rate is 1211.36 nGy/h, 20 times higher than the estimated average global primordial radiation of 60 nGy/h and 6 times higher than that of the world range (10-200 nGy/h). The radium equivalent (Ra eq ) values are from 6 to 9 times the recommended value. The internal and external hazard indices (H int , H ex ) indicate that their values are from 6 to 11 times the permissible values of these indices. These higher values may be due to the presence of economic heavy minerals containing radionuclides as zircon and monazite as well as some trace minerals, thorite and uranothorite. The mineralogical study indicates the beach sands contain heavy minerals, zircon, monazite, rutile, ilmenite, leucoxene, magnetite and garnet. The average abundance of zircon is 0.175 wt% ranging from 0.125 wt% to 0.239 wt%, while it is 0.004wt% ranging from 0.001 wt% to 0.007 wt% for monazite. The average abundance is 0.087 wt% for rutile; 2.029 wt% for ilmenite; 1.084 wt% for magnetite; 0.384 wt% for leucoxene and 0.295 wt% for garnet. Radiometric measurements were carried out for the beach sands from East Rosetta estuary to determine the activity concentrations of 238U, 226Ra, 232Th, and 40K, using a Hyper Pure Germanium spectrometer, to estimate the dose rates and radiation hazard indices. The average specific activities are 778.20 Bq/kg for 238U; 646.89 Bq/kg for 226Ra; 621.92 and 627.85 Bq/kg for the 222Rn daughters 214pb and 214Bi respectively. The average specific activity of 232Th is 1510.25 Bq/kg, while the calculated specific activity for 4-K has an average of 8.41 Bq/kg. The average specific activity of 235U is 38.61 Bq/kg. The average absorbed dose rate is 1211.36 nGy/h, 20 times higher than the estimated average global primordial radiation of 60 nGy/h and 6 times higher than that of the world range (10-200 nGy/h). The radium equivalent (Raeq) values are from 6 to 9 times the recommended value. The internal and external hazard indices (Hint, Hex) indicate that their values are from 6 to 11 times the permissible values of these indices. These higher values may be due to the presence of economic heavy minerals containing radionuclides as zircon and monazite as well as some trace minerals, thorite and uranothorite. The mineralogical study indicates the beach sands contain heavy minerals, zircon, monazite, futile, ilmenite, leucoxene, magnetite and garnet. The average abundance of zircon is 0.175 wt% ranging from 0.125 wt% to 0.239 wt%, while it is 0.004wt% ranging from 0.001 wt% to 0.007 wt% for monazite. The average abundance is 0.087 wt% for rutile; 2.029 wt% for ilmenite; 1.084 wt% for magnetite; 0.384 wt% for leucoxene and 0.295 wt% for garnet.
出处 《Chinese Journal Of Geochemistry》 EI CAS CSCD 2013年第2期146-156,共11页 中国地球化学学报
关键词 放射性核素 海滩砂 矿物学 核素测量 河口 平均丰度 埃及 辐射测量 Egyptian black sand gamma spectrometer radiation hazards 222Rn daughters economic heavy minerals
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参考文献37

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