期刊文献+

杭州市办公场所室内空气中PBDEs的污染现状与特征 被引量:7

Pollution Status and Characteristics of PBDEs in Indoor Air of Hangzhou
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摘要 分析评价了杭州市办公场所中PBDEs的污染现状、污染特征.结果表明,办公场所中PBDEs气相和颗粒相总浓度范围为40.66~141.00Pg·m^-2,平均浓度为93.22Pg·m^-2,是家庭室内、室外浓度的1.87、5.01倍.BDE-47、BDE-99为办公场所中最重要的两种同系物,分别占总浓度的33.29%、31.99%.PBDEs气相浓度是颗粒相的1.34倍,其中BDE-28、BDE-47、BDE-99主要存在于气相中,BDE-153、BDE-183主要存在于颗粒相中. Pollution Status and characteristics of PBDEs in offices were investigated in Hangzhou. As a result, the total concentration of PBDEs was 40. 66-141.00 pg.m-3 , and the mean concentration was 93.22 pg.m-3 , being 1.87 and 5.01 times as high as those in homes and outdoor. In particle and gas phases, BDE-47 and BDE-99 were the most abundant congeners, which accounted for 33.29% and 31.99% of total PBDEs, respectively. Concentration of PBDEs in gas phase was 1.34 times as high as that in particle phase. BDE-28, BDE-47 and BDE-99 mainly existed in the gas phase, while BDE-153 and BDE-183 mainly existed in the particle phase.
出处 《环境科学》 EI CAS CSCD 北大核心 2014年第1期41-45,共5页 Environmental Science
基金 国家自然科学基金项目(20977075) 国家高技术研究发展计划(863)项目(2010AA064901 2010AA064902) 浙江省重点科技创新团队项目(2009R50047)
关键词 多溴联苯醚 办公场所 室内空气 浓度水平 污染特征 polybrominated diphenyl ethers office indoor air concentrations pollution characteristics
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参考文献22

  • 1Hites R A. Polybrominated diphenyl ethers in the environment and in people: A met-analysis of concentrations [ J ]. Environmental Science & Technology, 2004, 38(4) : 945-956.
  • 2Alaee M, Arias P, Sjodin A, et al. An overview of commercially used brominated flame retardants, their applications, their use patterns in different countries/regions and possible modes of release [ J ]. Environment International, 2003, 29 ( 6 ) : 683- 689.
  • 3Osako M, Kim Y J, Ma K C. Leaching of brominated flame retardants in leaehate from landfills in Japan [ J]. Chemosphere, 2004, 57(10) : 1571-1579.
  • 4Yu Z Q, Zheng K W, Ren G F, et al. Identification of Monochloro-nonabromodiphenyl ethers in the air and soil samples from South China [ J ]. Environmental Science & Technology, 2011, 45(7) : 2619-2625.
  • 5Johnson P I, Stapleton H M, Mukherjee B, et al. Associations between brominated flame retardants in house dust and hormone levels in men [ J ]. Science of the Total Environment, 2013, 445: 177-184.
  • 6Shoeib M, Harner T, Webster G M, et al. Legacy and current- use flame retardants in house dust from Vancouver, Canada[ J]. Environmental Pollution, 2012, 169 : 175-182.
  • 7Muenhor D, Harrad S. Within-room and within-building temporal and spatial variations in concentrations of polybrominated diphenyl ethers (PBDEs) in indoor dust [ J ]. Environment International, 2012, 47 : 23-27.
  • 8Wang L C, Lee W J, Lee W S, et al. Polybrominated diphenyl ethers in various atmospheric environments of Taiwan: Their levels, source identification and influence of combustion sources [J]. Chemosphere, 2011, 84(7): 936-942.
  • 9Birnbaum L S, Staskal D F. Brominated flame retardants: Cause for concern[ J]. Environmental Health Perspectives, 2004, 112 (1):9-17.
  • 10Vorkamp K, Thomsen M, Frederiksen M, et al. Polybrominated diphenyl ethers (PBDEs) in the indoor environment and associations with prenatal exposure [ J ]. Environment International, 2011, 37(1): 1-10.

二级参考文献111

  • 1王庆一.中国能源现状与前景[J].中国煤炭,2005,31(2):22-27. 被引量:17
  • 2陈社军,麦碧娴,曾永平,罗孝俊,余梅,盛国英,傅家谟.珠江三角洲及南海北部海域表层沉积物中多溴联苯醚的分布特征[J].环境科学学报,2005,25(9):1265-1271. 被引量:117
  • 3姜志宽,王以燕.我国的卫生杀虫剂发展概况[J].中华卫生杀虫药械,2006,12(6):413-418. 被引量:34
  • 4杜雪晴,王新明,唐建辉,丁翔,林海涛,李忠,盛国英,傅家谟.我国主要市售香烟主流烟气中多环芳烃的分析[J].环境化学,2006,25(6):785-788. 被引量:19
  • 5Harrad S,Hazrati S,Ibarra C.Concentrations of polychlorinated biphenyls in indoor air and polybrominated diphenyl ethers in indoor air and dust in Birmingham,United Kingdom:Implications for human exposure.Environ Sci Technol,2006,40:4633-4638.
  • 6Allen J G,McClean M D,Stapleton H M,et al.Personal exposure to polybrominated diphenyl ethers (PBDEs) in residential indoor air.Environ Sci Technol,2007,41:4574-4579.
  • 7Lemieux P M,Lutes C C,Santoianni D A.Emissions of organic air toxics from open burning:A comprehensive review.Prog Enery Combust,2004,30:1-32.
  • 8Liu Y N,Tao S,Dou H,et al.Exposure of traffic police to polycyclic aromatic hydrocarbons in Beijing,China.Chemosphere,2007,66:1922-1928.
  • 9Cheng J P,Yuan T,Wu Q,et al.PM10-bound polycyclic aromatic hydrocarbons (PAHs) and cancer risk estimation in the atmosphere surrounding an industrial area of Shanghai,China.Water Air Soil Poll,2007,183:437-446.
  • 10Zhu L Z,Lu H,Chen S G,et al.Pollution level,phase distribution and source analysis of polycyclic aromatic hydrocarbons in residential air in Hangzhou,China.J Hazard Mater,2009,162:1165-1170.

共引文献74

同被引文献94

  • 1LUO XiaoJun,CHEN SheJun,MAI BiXian & FU JiaMo State Key Laboratory of Organic Geochemistry,Guangzhou Institute of Geochemistry,Chinese Academy of Sciences,Guangzhou 510640,China.Advances in the study of current-use non-PBDE brominated flame retardants and dechlorane plus in the environment and humans[J].Science China Chemistry,2010,53(5):961-973. 被引量:12
  • 2叶细标,傅华.多溴联苯醚的环境暴露及健康危害[J].环境与职业医学,2007,24(1):95-101. 被引量:34
  • 3王俊,张干,李向东,李军,钟流举,向运荣,彭永焯.珠江三角洲地区大气中多溴联苯醚的被动采样观测[J].中国环境科学,2007,27(1):10-13. 被引量:11
  • 4王旭.哈尔滨市土壤与大气中OCPs和BFRs分布特征及源汇分析[D].哈尔滨:哈尔滨工业大学环境工程学院,2009.
  • 5De Wit, Cynthia A. An overview of brominated flame retar- dants in the environment[J]. Chemosphere, 2002,46(5) : 583- 624.
  • 6周政懋.世界阻燃剂发展趋势探讨及国内产业现状分析[A].//中国阻燃学会.2009年中国阻燃学术年会论文集[c].中国阻燃学会,2009:21.
  • 7Tang, Hubert Po On. Recent development in analysis of persis- tent organic pollutants under the Stockholm Convention [J]. Trac Trends in Analytical Chemistry, 2013(45) :48-66.
  • 8F Reber Brown, Todd P Whitehead, Jone-soo Park, et al. Lev- els of non-polybrominated diphenyl ether brominated flame retardants in residential house dust samples and fire station dust samples in California[J]. Environmental Research, 2014 (135) :9-14.
  • 9Robin J Law,Adrian Covaci,Stuart Harrad,et al. Levels and trends of PBDEs and HBCDs in the global environment:status at the end of 2012 [J]. Environment International, 2014 (65) : 147-158.
  • 10Vincent J Decarlo. Studies on brominated chemicals in the en- viroment[J]. Annals of the New York Academy of Sciences, 1979,320( 1 ) :678-681.

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