摘要
Based on automatic continuous surface ozone concentration observation data from June 10, 2010 to March 20, 2012 in the Taklimakan Desert hinterland, combined with corresponding meteorological data, the temporal, seasonal and daily variation characteristics of surface ozone concentrations under different weather conditions were analyzed. At the same time, the main fac- tors affecting ozone variation are discussed. Results show that： （1） Daily variation of ozone concentration was characterized by one obvious peak, with gentle changes during the night and dramatic changes during the day. The lowest concentration was at 09：00 and the highest was at 18：00. Compared to urban areas, there was a slight time delay. （2） Ozone concentration variation had a weekend effect phenomenon. Weekly variation of ozone concentration decreased from Monday to Wednesday with the lowest in Wednesday, and increased after Thursday with the highest in Sunday. （3） The highest monthly average concentration was 89.6 I.tg/m3 in June 2010, and the lowest was 32.0 ~g/m3 in January 2012. Ozone concentration reduced month by month from June to December in 2010. （4） Ozone concentration in spring and summer was higher than in autumn and winter. The variation trend agreed with those in other large and medium-sized cities. （5） Under four different types of weather, daily ozone concentration var- ied most dramatically in sunny days, followed by slight variation in rain days, and varied gently in cloudy days. Ozone concentra- tion varied inconspicuously before a sandstorm appearance, and dropped rapidly at the onset of a sandstorm. （6） Daily variation of radiation was also characterized by a single peak, and the variation was significantly earlier than ozone concentration variation. Sun radiation intensity had a direct influence on the photochemical reaction speed, leading to variation of ozone concentration. （7） Daily average ozone concentration in dust weather was higher than in slight rain and clear days. The variation of near surface ozone concentration could also be affected by meteorological factors such as relative humidity, wind speed, wind direction and sunshine hours. Thus, numerous factors working together led to ozone pollution.
Based on automatic continuous surface ozone concentration observation data from June 10, 2010 to March 20, 2012 in the Taklimakan Desert hinterland, combined with corresponding meteorological data, the temporal, seasonal and daily variation characteristics of surface ozone concentrations under different weather conditions were analyzed. At the same time, the main fac- tors affecting ozone variation are discussed. Results show that： （1） Daily variation of ozone concentration was characterized by one obvious peak, with gentle changes during the night and dramatic changes during the day. The lowest concentration was at 09：00 and the highest was at 18：00. Compared to urban areas, there was a slight time delay. （2） Ozone concentration variation had a weekend effect phenomenon. Weekly variation of ozone concentration decreased from Monday to Wednesday with the lowest in Wednesday, and increased after Thursday with the highest in Sunday. （3） The highest monthly average concentration was 89.6 I.tg/m3 in June 2010, and the lowest was 32.0 ~g/m3 in January 2012. Ozone concentration reduced month by month from June to December in 2010. （4） Ozone concentration in spring and summer was higher than in autumn and winter. The variation trend agreed with those in other large and medium-sized cities. （5） Under four different types of weather, daily ozone concentration var- ied most dramatically in sunny days, followed by slight variation in rain days, and varied gently in cloudy days. Ozone concentra- tion varied inconspicuously before a sandstorm appearance, and dropped rapidly at the onset of a sandstorm. （6） Daily variation of radiation was also characterized by a single peak, and the variation was significantly earlier than ozone concentration variation. Sun radiation intensity had a direct influence on the photochemical reaction speed, leading to variation of ozone concentration. （7） Daily average ozone concentration in dust weather was higher than in slight rain and clear days. The variation of near surface ozone concentration could also be affected by meteorological factors such as relative humidity, wind speed, wind direction and sunshine hours. Thus, numerous factors working together led to ozone pollution.
基金
supported by Natural Science Foundation of China(Nos.41175017,41175140)
China Special Fund for Meteorological Research in the Public Interest(Nos.GYHY201006012,GYHY201106025)
