摘要
Luminescence intensity of CdS：Mn/ZnS core-shell quantum dots （QDs） can be strongly enhanced in comparison with bulk CdS：Mn and nanoparticles, while the luminescence due to the surface state is greatly suppressed by a capping ZnS shell We find that with the increasing temperature, the peak position of CdS：Mn/ZnS core-shell QDs blue shifts due to the reduction of phonon coupling. Unlike the bulk CdS：Mn, the luminescence of the core-shell QDs is less sensitive to thermal quenching.
Luminescence intensity of CdS：Mn/ZnS core-shell quantum dots （QDs） can be strongly enhanced in comparison with bulk CdS：Mn and nanoparticles, while the luminescence due to the surface state is greatly suppressed by a capping ZnS shell We find that with the increasing temperature, the peak position of CdS：Mn/ZnS core-shell QDs blue shifts due to the reduction of phonon coupling. Unlike the bulk CdS：Mn, the luminescence of the core-shell QDs is less sensitive to thermal quenching.
基金
Supported by the National Natural Science Foundation of China under Grant Nos 11074232, 11274288 and 21002097, the National Basic Research Program of China under Grant Nos 2011CB932801 and 2012CB933702, and the Specialized Research Fund for the Doctoral Program of Higher Education of China under Grant No 20123402110034.
