期刊文献+

雨季广州大气中的硝酸盐粒子(英文) 被引量:1

Nitrate Particles in the Air of Guangzhou during Rainy Season
下载PDF
导出
摘要 对雨季广州大气中的硝酸盐粒子进行了两年的观察 .粒子被分为两部分 :粗大粒子 (r >1.0 μm )和微小粒子 (r≤ 1.0 μm ) .用离子色谱对粒子总量进行了总体分析 ,用复合薄膜法和X_射线分析法对单个粒子进行了分析 .总体分析结果表明 ,粗大粒子中的NO- 3、Ca2 +和Na+含量比微小粒子中的高 .对单个粒子的分析发现 ,硝酸盐粒子不仅存在于粗大粒子中 ,而且也存在于微小粒子中 ,证明硝酸能凝结在海盐上形成粗大硝酸盐粒子 ,粗大硝酸盐粒子有可能起着最终消除广州大气中硝酸的作用 . Aerosol samples were collected from the air of Guangzhou during rainy season for two years. Atmospheric particles were size_fractionated into two size ranges: coarse particles( r >1.0 μm) and fine particles ( r ≤1.0 μm). The aerosol particles were measured with bulk analyses by ion chromatography and analyses of individual particles by multiple thin film method and X_ray analysis technique. Chemical analysis of bulk samples showed that the content of NO - 3, Ca 2+ and Na + in the coarse size range was much higher than that in the fine size range. Analyses of individual particle showed that nitrate particles existed not only in the coarse size range but also in the fine size range. Evidence of nitric acid condensed on the sea salt particle to form a coarse nitrate particle was obtained. Coarse nitrate particles probably serve as a permanent removal mechanism for nitric acid in the air of Guangzhou during rainy season.
出处 《华南理工大学学报(自然科学版)》 EI CAS CSCD 北大核心 2002年第1期84-88,共5页 Journal of South China University of Technology(Natural Science Edition)
基金 国家自然科学基金资助项目 (2 0 0 770 0 9) 广东省环境保护局和高等教育厅科技研究开发项目 (B2 30 2 5 6 4 ) 广州市环境保护局资助项目 (30 2_B2 6 980 )~~
关键词 硝酸盐粒子 复合薄膜法 广州 雨季 X-射线分析法 大气观测 粗大粒子 微小粒子 nitrate individual particle multiple thin film method Guangzhou rainy season
  • 相关文献

参考文献11

  • 1Spicer C W,Schumacher PM.Particulate nitrate laboratory and field studies of major sampling interfe-rence[J].Atmospheric Environment,1979, 13(3):543-552.
  • 2Qian G W,Ishizaka Y,Tsuruta H.Chemical change of aerosol particles during theformation of acidic fog droplets [J].J Chem Soc(in Japanese),1991,1991(5):690-697.
  • 3Qian G W,Ishizaka Y.Electron microscope studies of methane sulfonic acid inindividual aerosol particles [J].J Geophys Res,1993,98:8 459-8 470.
  • 4Junge C E.Air chemistry and radioactivity [M].New York:Academic Press, 1963.
  • 5Stelson A W,Friedlander S K,Seinfeld J H.A note on the equilibrium relationshipbetween ammonia and nitric acid and particulate ammonium nitrate [J].AtmosphericEnvironment,1979,13(2):369-371.
  • 6Qian G W,Ishizaka Y,Minami Y,et al.Transformation of individual aerosol particlesin acidic fog evolution [J].J Meteorol Soc(in Japanese), 1992,70(7):711-722.
  • 7Lan S H,Qian G W.Nitrate particles in the air of Guangzhou during dry season [J].Jof South China Univ of Tech (Natural Science Edition),2001,29(2):104-107.
  • 8Qian G W,Ishizaka Y.Analysis of individual particles using thin film method [J].JAerosol Research(in Japanese),1993,8(2):106-111.
  • 9Bigg E K,Ono A,Williams J.Chemical tests for individual submicron aerosol particles[J].Atmospheric Environment,1974,8(1):1-13.
  • 10Tang I N.Phase transformation and growth of aerosol particles composed of mixedsalts [J].J Aerosol Soc(in Japanese),1976,7:361-371.

同被引文献28

  • 1钱公望,刘焕彬.广州大气粒子中的硝酸和硫酸离子[J].华南理工大学学报(自然科学版),1997,25(10):94-98. 被引量:7
  • 2辞海编辑委员会.辞海[M].上海:上海辞书出版社,2000..
  • 3大气科学名词审定委员会.大气科学名词[M].北京:科学出版社,1996.2409.
  • 4Qian G W,Hu Y.Concentration of aerosol particles above and bellow a Casuarina Equisenfifolia forest canopy[C]//Liu Huaniin,Zhan Huaiyu,Xie Yimin.Emerging Technologies off Pulping & Papermaking of Fast-Growing Wood:ISETPP98.Guangzhou:Publishing company of South China University of Technology,1998:390-394.
  • 5Ishzaka Y,Qian G W.Sampling of nitrate particles in the air of Guangzhou[J].Proc M S J Annu Meet,1999,77(2):312-313.
  • 6Qian G W,Hu J,Shi X L.Deposition of acidic particles to Casuarina Equisetifolia forest[C]// Liu Huanbin,Zhan Huaiyu,Xie Yimin.Emerging Technologies of Pulping & Papermaking of Fast-Growing Wood:2nd ISETPP.Guangzhou:Publishing Company of South China University of Technology,2002:159-161.
  • 7钱公望.测定单个大气气溶胶微粒的初步研究[C]//第二届环境化学中青年学者学术研讨会.广州:华南理工大学出版社,2003:31-33.
  • 8Waller R E,Brooks A G F,Cartwright J.An electron microscope study of particles in town air[J].Int J Air Water Pollut,1963 (7):779-786.
  • 9Junge C E.Air chemistry and radioactivity[M].New York:Academic Press,1963.
  • 10Yamato M,Iwasaka Y,Qian G W,et al.Sulfuric acid as background aerosols over oceans in southern hemisphere and surrounding Antarctica[J].Aerosol Sci Tech Japan,1988(6):85-88.

引证文献1

二级引证文献10

相关作者

内容加载中请稍等...

相关机构

内容加载中请稍等...

相关主题

内容加载中请稍等...

浏览历史

内容加载中请稍等...
;
使用帮助 返回顶部