摘要
本文将我们建立的非相干光时延四波混频(TDFWM-IL)的多能级理论由均匀加宽情形发展到非均匀加宽情形,得到吸收带同时存在均匀和非均匀加宽时,TDFWM-IL多能级理论给出的信号强度随两束泵光相对延时的一般关系式,讨论非均匀加宽占绝对优势时,非相干光光子回波的多能级理论结果,及其与二能级理论结果的差异,论证等效二能级模型同样适用于近似分析存在非均匀加宽影响时,吸收带TDFWM-IL的实验结果,报道在红宝石零声子线和甲酚紫固体膜吸收边上的实验结果,并与上述理论做了比较。
In this paper, our multi-level theory of time-delay four wave mixing with incoherent light (TDFWM-IL) developed previously for the case of homogeneous broadening system has been extended to a generally inhomogeneous broadening case. From the present theory, a general expression of signal intensity for absorption band with both homogeneous and inhomogeneous broadening is given as a function of mutual time delay τ between two pump beams. Photon echo with incoherent light under the condition of extremely inhomogeneous broadening is discussed, and the difference of results obtained scperately from multi-level and two-level theory is pointed out. It has been demonstrated that the experiment of TDFWM-IL can also be analysed approximately by using an effective two-level model when a weak effect of inhomogeneous broadening of absorption band exists. Finally, our experimental results of TDFWM-IL obtained at zero-phonon line of ruby and absorption edge of cresyl violet film in PMMA are also presented and compared with the theory mentioned above.
出处
《物理学报》
SCIE
EI
CAS
CSCD
北大核心
1991年第3期414-423,共10页
Acta Physica Sinica