摘要
设计了一种全新的测量搅拌釜内动态体系温度、压力的设备及方案,以CO2-H2O体系为特征体系,对搅拌状态下气液二相动态相对稳定状态进行了研究。搅拌釜内流体发生湍动,达到相平衡的气液二相的传质极限发生偏移。在不同温度(288.15—307.15 K)和转速(190—520 r/min)下进行实验,温度一定时,动态平衡偏移率随湍动程度的增大而增大。温度为307.15 K、转速为520 r/min时,动态平衡偏移率高达27%。利用动态平衡偏移率反算搅拌釜内的雷诺数ReD,将其与传统计算得出的雷诺数ReT进行比较拟合得到关联式。
A stirred vessel which is capable of measuring dynamic temperature and pressure of the system was designed to study the dynamic relative steady state of turbulent CO2-H2O system. The mass transfer limitation deviates when gas-liquid system of static mass transfer equilibrium begins to flow. The experiments at different temperatures (288.15--307.15 K) and speeds (190--520 r/min) show that strengthening turbulence of fluid can increase the deviation. When temperature is 307.15 K, speed is 520 r/min, the dynamic equilibrium deviation rate r is as high as 27%. Processing data and Re_D can be calculated by the relationship of Re and r. The correlation of ReD and ReT is gained by fitting experimental data.
出处
《化学工程》
CAS
CSCD
北大核心
2015年第5期49-52,67,共5页
Chemical Engineering(China)
关键词
气液传质
搅拌
流体湍动
动态传质平衡
雷诺数
gas-liquid mass transfer
stir
fluid turbulence
dynamic mass transfer equilibrium
Reynolds number