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折板光催化反应器降解甲醛效果测试

FORMALDEHYDE REMOVING PERFORMANCE IN FOLDED-PLATE PHOTOCATALYTIC REACTOR
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摘要 采用对比法测试不同结构折板反应器光催化降解甲醛的效果,并用CFD软件对流速场和降解效率进行模拟计算。研究表明:折板反应器能增大反应面积和紫外光入射角,平衡传质.反应能力,与平板型相比,广角型和窄角型折板反应器的降解效率分别提高1.5倍和1.9倍;CFD模拟说明折板反应器内竖直方向流速分布均匀,但水平方向和薄板表面分布不均,影响对流传质效果;与实测数据相比,模拟计算结果高出6.4%~15.1%,但两者变化趋势相同;并且反应器内湿度过高会降低降解效率。 The comparing method was used to test the effect of photocatalytic degradation of formaldehyde for folded- plate reactors with different structures, and CFD software was used to simulate and calculate the velocity field and the degradation efficiency. The results showed that the folded-plate reactor can enlarge reaction area and UV incidence angle, balance mass transfer-reaction capability. Comparing with plate reactor, the degradation efficiencies in wide- angle and narrow-angle folded-plate reactors increase 50% and 90%, respectively. The computational fluid dynamics (CFD) simulation showed that the distribution of flow velocity is uniform in vertical direction and uneven in horizontal direction and surface of thin plate of the folded-plate reactor, affecting convective mass transfer effect. The simulation results are higher than testing data by 6.4%- 15.1%, however, their change trend is same. Moreover, the degradation efficiency will be decreased if the humidity is too high in reactor.
作者 刘鹏 郑洁
出处 《太阳能学报》 EI CAS CSCD 北大核心 2015年第12期3103-3107,共5页 Acta Energiae Solaris Sinica
基金 国家"十二五"科技支撑计划(2011BAJ03B13)
关键词 光催化氧化 折板反应器 甲醛 CFD模拟 photocatalytic oxidation folded-plate reactor formaldehyde CFD simulation
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参考文献12

  • 1Zhang Jiefeng, Bai Zhipeng, Chang Victor W C, et al. Balancing BEC and IAQ in civil buildings during rapid urbanization in China : Regulation, interplay and collaboration[J]. Energy Policy, 2011, 39(10): 5778-5790.
  • 2Wesehler C J. Changes in indoor pollutants since the 1950s[J]. Atmospheric Environment, 2009, 43(1) : 153-169.
  • 3Aydogan A, Montoya L D. Formaldehyde removal by common indoor plant species and various growing media [J]. Atmospheric Environment, 2011, 45 (16) : 2675- 2682.
  • 4Destaillats H, Sleiman M, Sullivan D P. Key parameters influencing the performance of photoeatalytie oxidation (PCO) air purification under realistic indoor conditions [J]. Applied Catalysis B: Environmental, 2012, 128: 159-170.
  • 5Zhong Lexuan, Haghighat F, Blondeau P, et al. Modeling and physical interpretation of photoeatalytie oxidation efficiency in indoor air applications[J]. Building and Environment, 2010, 45 (12) : 2689- 2697.
  • 6王德峥.Langmuir-Hinshelwood动力学的有效实验条件(英文)[J].催化学报,2010,31(8):972-978. 被引量:6
  • 7中国家用电器研究院等.GB/T18801-2008空气净化器[S],2008.
  • 8Mo Jinhan, Zhang Yinping, Xu Qiujian, et al. Photocatalytic purification of volatile organic compounds in indoor air: A literature review[J]. Atmospheric Environment, 2009, 43(14): 2229-2246.
  • 9Passalia C, Alfano O M, Brandi R J. A methodology for modeling photocatalytic reactors for indoor pollution control using previously estimated kinetic parameters [J]. Journal of Hazardous Materials, 2012, 211-212: 357-365.
  • 10Mo Jinhan, Zhang Yinping, Yang Rui, et al. Influence of fins on formaldehyde removal in annular photocatalytic reactors [J]. Building and Environment, 2008, 43(3) : 238-245.

二级参考文献35

  • 1Froment G F,Bischoff K B.Chemical Reactor Analysis and Design.2nd Ed.New York:Wiley,1990.70.
  • 2Boudart M.Kinetics of Chemical Processes.New Jersey:Prentice-Hall,1968 (reprinted:Boston:Butterworth-Heinemann,1991).63.
  • 3Segel I H.Enzyme Kinetics:Behavior and Analysis of Rapid Equilibrium and Steady State Enzyme Systems.New York:Wiley,1993.29.
  • 4Espenson J H.Chemical Kinetics and Reaction Mechanism.2nd Ed.New York:McGraw-Hill,1995.78,87.
  • 5Vincent R S,Lindstedt R P,Malika N A,Reid I A B,Messenger B E.J Catal,2008,260:37.
  • 6Heineken F G,Tsuchiya H M,Aris R.Math Biosci,1967,1:95.
  • 7Moore J W,Pearson R G.Kinetics and Mechanism.3rd Ed.New York:Wiley,1981.314.
  • 8Steinfeld,J I,Francisco J S,Hase W L.Chemical Kinetics and Dynamics.2nd Ed.New Jersey:Prentice Hall,1999.39.
  • 9Tomlin A S,Turányi T,Pilling M J.In:Pilling M J ed.Low-Temperature Combustion and Autoignition,Comprehensive Chemical Kinetics.Vol.35.Amsterdam:Elsevier,1997.380.
  • 10Kapteijn F,Berger R J,Moulijn J A.In:Ertl G,Knozinger H,Schuth F,Weitkamp J eds.Handbook of Heterogeneous Catalysis.2nd Ed.Vol.3.Weinheim:Wiley-VCH,2008.1696.

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