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Decoherence-and Dimerization-assisted Energy Transport in Protomer of Light-Harvesting Complexes

Decoherence-and Dimerization-assisted Energy Transport in Protomer of Light-Harvesting Complexes
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摘要 We have investigated the dynamics of a protomer coupled to two different decoherent environments,each in a configuration called the spin star configuration.Using the quantum mechanics method,in different situations,we obtain the analytical expressions for the transition probability in the protomer system.In thermal equilibrium,there exist well-defined ranges of parameters for which decoherent interaction between the protomer and the environment assists energy transfer in the protomer system,while in pure quantum mechanics states,the decoherent interaction assists energy transfer for an eigenstate but against energy transfer for quantum mechanics averages.In particular,we also find that the dimerization of two bacteriochlorophylls in protomer can always assist energy transfer in certain parameter range,and in the appropriate spin bath energy,the efficiency of energy transport is sensitively depended on the temperature of environments.
出处 《Communications in Theoretical Physics》 SCIE CAS CSCD 2016年第1期114-120,共7页 理论物理通讯(英文版)
基金 Supported by the National Natural Science Foundation of China under Grant Nos.11274272,11304281,31201001 by the Natural Science Foundation of Zhejiang Province under Grant Nos.Y6110250 LY14A040001 and Zhejiang Ocean University(X12ZD10)
关键词 clecoherence assisted energy transport light-harvesting complexes protomer 二聚化 退相干 捕光复合物 能源运输 亚基 相互作用参数 环境温度 量子力学
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