摘要
将二氧化碳(CO_2)催化加氢转化为具有高附加值的烃类化合物,既可减缓大气中CO_2浓度的攀升速度,又符合可持续发展战略,对环境和社会均具有重要意义。本文综述了Fe基催化剂上CO_2加氢制C_2+烃的研究进展,着重介绍了反应路径及机理、催化剂研制及反应器设计,展望了CO_2制烃的研究前景。
Catalytic conversion of carbon dioxide（ CO2） to value-added hydrocarbons is of great environmental and social importance,which can not only reduce CO2 concentration in the atmosphere,but also conform with sustainable development strategy. This paper reviews the progress in catalytic conversion of CO2 to C2＋hydrocarbons over Fe-based catalyst. Reaction pathway and mechanism,catalyst preparation and reactor design are emphatically introduced. In addition,the future of hydrocarbons synthesis via CO2 hydrogenation is also summarized.
出处
《应用化学》
CAS
CSCD
北大核心
2016年第2期123-132,共10页
Chinese Journal of Applied Chemistry
基金
国家自然科学基金资助项目(21503029,21503027)
中央高校基本科研业务费专项资金资助(DUT15ZD236,DUT15RC(3)027)
关键词
二氧化碳
催化加氢
Fe基催化剂
烃类合成
carbon dioxide
hydrogenation
Fe-based catalyst
hydrocarbons synthesis
