摘要
花岗岩作为高放废物处置库的地质屏障,其所含裂隙形成大量"通道"为废物在地下水运移提供条件,研究其迁移规律可为管控高放废物等问题提供理论数据。试验使用自制花岗岩裂隙溶质迁移试验设备,进行了以Na、Cu、U为示踪剂的迁移试验,得出以下结论:(1)裂隙中各示踪剂随迁移距离增加,相对浓度峰值逐渐减小,峰面积逐渐增大,时间-相对浓度曲线"缩首"现象减弱且"拖尾"现象明显;(2)对比三种示踪剂迁移曲线发现,曲线"缩首"现象程度U〉Na〉Cu,曲线"拖尾"现象程度Cu〉Na〉U;推测出花岗岩对三种示踪剂阻滞作用Cu〉Na〉U;(3)使用配线法分别求出Na、Cu、U的纵向弥散度分别为:0.084 2~0.107 7m、0.092 1~0.116 2m、0.095 8~0.133 7m;横向弥散度为:0.000 77m、0.000 66m、0.000 30m。
High-level radioactive waste would transport into groundwater by a large number of"channels"in the granite fracture.The study of the migration law can provide theoretical data for control of high-level waste.The following experiments were designed and carried out:Na,Cu and U transport experiment in granite rock.The experimental results show that:(1)With increasing distance,the concentration of peak value is decreasing and tailing phenomena is more obvious;(2)The maximum degree of tailing phenomena is curve of Cu and minimum degree of tailing phenomena is curve of U;(3)Longitudinal disperse coefficient for Na,Cu and U in granite rock range from 0.084 2 mto 0.107 7 m,from0.092 1mto 0.116 2mand from 0.095 8mto 0.133 7mrespectively.Meanwhile,transverse dispersion coefficient for Na,Cu and U respectively is 0.000 77 m,0.000 66 m,0.000 30 m.
出处
《核化学与放射化学》
CAS
CSCD
北大核心
2016年第2期123-128,共6页
Journal of Nuclear and Radiochemistry
基金
国家自然科学基金资助项目(D010901)
江西省自然科学基金资助项目(20122BAB206001)