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Theoretical study on non-sequential double ionization of carbon disulfide with different bond lengths in linearly polarizedlaser fields

Theoretical study on non-sequential double ionization of carbon disulfide with different bond lengths in linearly polarizedlaser fields
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摘要 By using a two-dimensional Monte-Carlo classical ensemble method, we investigate the double ionization(DI) process of the CS_2 molecule with different bond lengths in an 800-nm intense laser field. The double ionization probability presents a "knee" structure with equilibrium internuclear distance R = 2.9245 a.u.(a.u. is short for atomic unit). As the bond length of CS increases, the DI probability is enhanced and the "knee" structure becomes less obvious. In addition,the momentum distribution of double ionized electrons is also investigated, which shows the momentum mostly distributed in the first and third quadrants with equilibrium internuclear distance R = 2.9245 a.u. As the bond length of CS increases,the electron momentum becomes evenly distributed in the four quadrants. Furthermore, the energy distributions and the corresponding trajectories of the double-ionized electrons versus time are also demonstrated, which show that the bond length of CS in the CS_2 molecule plays a key role in the DI process. By using a two-dimensional Monte-Carlo classical ensemble method, we investigate the double ionization(DI) process of the CS_2 molecule with different bond lengths in an 800-nm intense laser field. The double ionization probability presents a "knee" structure with equilibrium internuclear distance R = 2.9245 a.u.(a.u. is short for atomic unit). As the bond length of CS increases, the DI probability is enhanced and the "knee" structure becomes less obvious. In addition,the momentum distribution of double ionized electrons is also investigated, which shows the momentum mostly distributed in the first and third quadrants with equilibrium internuclear distance R = 2.9245 a.u. As the bond length of CS increases,the electron momentum becomes evenly distributed in the four quadrants. Furthermore, the energy distributions and the corresponding trajectories of the double-ionized electrons versus time are also demonstrated, which show that the bond length of CS in the CS_2 molecule plays a key role in the DI process.
作者 Kai-Li Song Wei-Wei Yu Shuai Ben Tong-Tong Xu Hong-Dan Zhang Pei-Ying Guo Jing Guo 宋凯莉;于伟威;贲帅;徐彤彤;张宏丹;郭培莹;郭静(Institute of Atomic and Molecular Physics,Jilin University;School of Physics and Electronic Technology,Liaoning Normal University)
出处 《Chinese Physics B》 SCIE EI CAS CSCD 2017年第2期176-182,共7页 中国物理B(英文版)
基金 Project supported by the National Natural Science Foundation of China(Grant Nos.11574117 and11604131)
关键词 intense laser field non-sequential double ionization classical ensemble method the bond length intense laser field non-sequential double ionization classical ensemble method the bond length
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