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Synthesis of ZnGaNO solid solution–carbon nitride intercalation compound composite for improved visible light photocatalytic activity

Synthesis of ZnGaNO solid solution–carbon nitride intercalation compound composite for improved visible light photocatalytic activity
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摘要 Visible-light-driven ZnGaNO solid solution–carbon nitride intercalation compound(CNIC) composite photocatalyst was synthesized via a mixing and heating method. The composite photocatalyst was characterized by X-ray diffraction(XRD), field-emission scanning electron microscopy(FESEM), high-resolution transmission electron microscopy(HRTEM), Fourier transform infrared(FT-IR) spectroscopy, UV-vis diffuse reflection spectroscopy, X-ray photoelectron spectroscopy(XPS), photoluminescence(PL) spectroscopy and BET surface area measurements. The activity of ZnGaNO–CNIC composite photocatalyst for photodegradation of methyl orange(MO) is higher than that of either single-phase CNIC or ZnGaNO solid solution. The as-prepared composite photocatalysts exhibit an improved photocatalytic activity due to enhancement for the separation and transport of photo-generated electron–hole pairs. Visible-light-driven ZnGaNO solid solution-carbon nitride intercalation compound (CNIC) composite photocatalyst was synthesized via a mixing and heating method. The composite photocatalyst was characterized by X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), Fourier transform infrared (FT-IR) spectroscopy, UV-vis diffuse reflection spectroscopy, X-ray photoelectron spectroscopy (XPS), photoluminescence (PL) spectroscopy and BET surface area measurements. The activity of ZnGaNO-CNIC composite photocatalyst for photodegradation of methyl orange (MO) is higher than that of either single-phase CNIC or ZnGaNO solid solution. The as-prepared composite photocatalysts exhibit an improved photocatalytic activity due to enhancement for the separation and transport of photo-generated electron-hole pairs.
出处 《Journal of Central South University》 SCIE EI CAS CSCD 2017年第2期276-283,共8页 中南大学学报(英文版)
基金 Project(51208102)supported by the National Natural Science Foundation of China
关键词 PHOTOCATALYSIS carbon nitride intercalation compound (CNIC) ZnGaNO COMPOSITE 复合光催化剂 光催化活性 氮化碳 插层化合物 合成 场发射扫描电子显微镜 X射线光电子能谱 漫反射光谱
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