摘要
钍基核燃料后处理Thorex流程的发展倾向于酸式进料,单循环。基于30级10mm环隙式离心萃取器台架系统,对酸式进料、单循环Thorex流程工艺进行台架实验验证。实验结果表明:全流程钍回收率为99.994%,铀回收率为99.30%,钍中去铀分离因子SF_(U/Th)为1.5×10~2,铀中去钍分离因子SF_(Th/U)为2.2×10~4。增加1B工艺段(钍铀分离段)补萃级数应可以进一步提高铀回收率。
The one-cycle acid Thorex process is recommended for thorium-based fuel reprocessing.Experimental verification of Thorex process was performed by 30 stages10 mm centrifugal extractors.The results show that the recovery of Th and U are 99.994% and 99.30% ,respectively.The SF_(U/Th) and SF_(Th/U) are 1.5×10~2 and 2.2×10~4,respectively.A higher recovery of U should be attained if the stages for supplement extraction of 1 Bsection are increased.
出处
《核化学与放射化学》
CAS
CSCD
北大核心
2018年第1期23-29,共7页
Journal of Nuclear and Radiochemistry
基金
中国科学院战略性先导科技专项--钍基熔盐堆核能系统(XDA02030000)
关键词
钍基核燃料
后处理
Thorex流程
离心萃取器
thorium-based nuclear fuel
reprocessing
Thorex process
centrifugal extractor