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Magnetic-field enhanced high-thermoelectric performance in topological Dirac semimetal Cd3As2 crystal 被引量:5

Magnetic-field enhanced high-thermoelectric performance in topological Dirac semimetal Cd_3As_2 crystal
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摘要 Thermoelectric materials can be used to convert heat to electric power through the Seebeck effect. We study magneto-thermoelectric figure of merit(ZT) in three-dimensional Dirac semimetal Cd_3As_2 crystal.It is found that enhancement of power factor and reduction of thermal conductivity can be realized at the same time through magnetic field although magnetoresistivity is greatly increased. ZT can be highly enhanced from 0.17 to 1.1 by more than six times around 350 K under a perpendicular magnetic field of 7 T. The huge enhancement of ZT by magnetic field arises from the linear Dirac band with large Fermi velocity and the large electric thermal conductivity in Cd_3As_2. Our work paves a new way to greatly enhance the thermoelectric performance in the quantum topological materials. Thermoelectric materials can be used to convert heat to electric power through the Seebeck effect. We study magneto-thermoelectric figure of merit (ZT) in three-dimensional Dirac semimetal Cd3A 5 2 crystal. It is found that enhancement of power factor and reduction of thermal conductivity can be realized at the same time through magnetic field although magnetoresistivity is greatly increased. ZT can be highly enhanced from 0.17 to 1.1 by more than six times around 350 K under a perpendicular magnetic field of 7 T. The huge enhancement of ZT by magnetic field arises from the linear Dirac band with large Fermi velocity and the large electric thermal conductivity in CdsA 5 2. Our work paves a new way to greatly enhance the thermoelectric performance in the quantum topological materials.
出处 《Science Bulletin》 SCIE EI CSCD 2018年第7期411-418,共8页 科学通报(英文版)
基金 supported by the National Key R&D Program of the Ministry of Science and Technology China(2017YFA0303001,2016YFA0300201 and 2017YFA0204904) the National Natural Science Foundation of China(11534010,11774325 and21603210) the Key Research Program of Frontier Sciences CAS(QYZDY-SSW-SLH021) Hefei Science Center CAS(2016HSCIU001) the Fundamental Research Funds for the Central Universities Supercomputing Center at USTC for providing the computing resources partially performed on the Superconducting Magnet and PPMS-16T Facilities,High Magnetic Field Laboratory of CAS
关键词 垂直磁场 半金属 热电 拓扑 水晶 性能 CDSA 热传导性 Dirac semimetal Thermoelectric material Magnetic field Enhancement of figure of merit
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