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Discovery of Two-Dimensional Quantum Spin Hall Effect in Triangular Transition-Metal Carbides

Discovery of Two-Dimensional Quantum Spin Hall Effect in Triangular Transition-Metal Carbides
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摘要 Though the quantum spin Hall effect(QSHE) in two-dimensional(2 D) crystals has been widely explored, the experimental realization of quantum transport properties is only limited to HgTe/CdTe or InAs/GaSb quantum wells. Here we employ a tight-binding model on the basis of d(z^2), d(xy), and d(x^2-y^2) orbitals to propose QSHE in the triangular lattice, which are driven by a crossing of electronic bands at the Γ point. Remarkably, 2 D oxidized Mxenes W2 M2 C3 are ideal materials with nontrivial gap of 0.12 eV, facilitating room-temperature observations in experiments. We also find that the nontrivially topological properties of these materials are sensitive to the cooperative effect of the electron correlation and spin-orbit coupling. Due to the feasible exfoliation from its 3 D MAX phase, our work paves a new direction towards realizing QSHE with low dissipation. Though the quantum spin Hall effect(QSHE) in two-dimensional(2 D) crystals has been widely explored, the experimental realization of quantum transport properties is only limited to HgTe/CdTe or InAs/GaSb quantum wells. Here we employ a tight-binding model on the basis of d(z^2), d(xy), and d(x^2-y^2) orbitals to propose QSHE in the triangular lattice, which are driven by a crossing of electronic bands at the Γ point. Remarkably, 2 D oxidized Mxenes W2 M2 C3 are ideal materials with nontrivial gap of 0.12 eV, facilitating room-temperature observations in experiments. We also find that the nontrivially topological properties of these materials are sensitive to the cooperative effect of the electron correlation and spin-orbit coupling. Due to the feasible exfoliation from its 3 D MAX phase, our work paves a new direction towards realizing QSHE with low dissipation.
作者 Shou-juan Zhang Wei-xiao Ji Chang-wen Zhang Shu-feng Zhang Ping Li Sheng-shi Li Shi-shen Yan 张守娟;纪维霄;张昌文;张树峰;李萍;李胜世;颜世申(School of Physics and Technology, University of Jinan;School of Physics, State Key Laboratory of Crystal Materials, Shandong University)
出处 《Chinese Physics Letters》 SCIE CAS CSCD 2018年第8期83-87,共5页 中国物理快报(英文版)
基金 Supported by the Natural Science Foundation of Shandong Province under Grant No ZR2018MA033 the National Natural Science Foundation of China under Grant No 11274143
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