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Measurement of Liquid Concentration Fields Near Interface with Cocurrent Gas-Liquid Flow Absorption Using Holographic Interferometry

Measurement of Liquid Concentration Fields Near Interface with Cocurrent Gas-Liquid Flow Absorption Using Holographic Interferometry
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摘要 Real-time laser holographic interferometry was applied to measure liquid concentrations of CO2 in the vicinity of gas-liquid free interface under the conditions of cocurrent gas-liquid flow for absorption of CO2 by ethanol. The influences of the Reynolds number on the measurable interface concentration and on the film thickness were discussed. The results show that CO2 concentration decreases exponentially along the mass transfer direction, and the concentration gradient increases as Reynolds number of either liquid or gas increases. CO2 concentrations fluctuate slightly along the direction of flow; on the whole, there is an increase in CO2 concentration. The investiga- tion also demonstrated that film thickness decreases with the increase of Reynolds number of either of the two phases. Sherwood number representing the mass transfer coefficient was finally correlated as a function of the hy- drodynamic parameters and the physical properties. Real-time laser holographic interferometry was applied to measure liquid concentrations of CO2 in the vicinity of gas-liquid free interface under the conditions of cocurrent gas-liquid flow for absorption of CO2 by ethanol. The influences of the Reynolds number on the measurable interface concentration and on the film thickness were discussed. The results show that CO2 concentration decreases exponentially along the mass transfer direction, and the concentration gradient increases as Reynolds number of either liquid or gas increases. CO2 concentrations fluctuate slightly along the direction of flow; on the whole, there is an increase in CO2 concentration. The investiga- tion also demonstrated that film thickness decreases with the increase of Reynolds number of either of the two phases. Sherwood number representing the mass transfer coefficient was finally correlated as a function of the hy- drodynamic parameters and the physical properties.
出处 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2006年第6X期747-753,共7页 中国化学工程学报(英文版)
基金 the National Natural Science Foundation of China (No.20476072)
关键词 cocurrent GAS-LIQUID flow ABSORPTION concentration field NEAR INTERFACE HOLOGRAPHIC INTERFEROMETRY cocurrent gas-liquid flow, absorption, concentration field, near interface, holographic interferometry
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参考文献3

  • 1J. Baranski,E. Bich,E. Vogel,J. K. Lehmann. Determination of Binary Diffusion Coefficients of Gases Using Holographic Interferometry in a Loschmidt Cell[J] 2003,International Journal of Thermophysics(5):1207~1220
  • 2A. M. Kutepov,B. G. Pokusaev,D. A. Kazenin,S. P. Karlov,A. V. Vyaz’min. Interfacial Mass Transfer in the Liquid–Gas System: An Optical Study[J] 2001,Theoretical Foundations of Chemical Engineering(3):213~216
  • 3L. M. Wolff,T. J. Hanratty. Instantaneous concentration profiles of oxygen accompanying absorption in a stratified flow[J] 1994,Experiments in Fluids(6):385~392

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