摘要
在高浓铀年龄的测量过程中,涉及到U、Pa的分离提取。本工作以天然铀、自制^(233)Pa为指示剂,研究了HCl、HF浓度等对TEVA树脂吸附U、Pa的影响,建立了TEVA色层法分离提取U和Pa的方法。结果表明:Pa的放化收率为99%,对Pa的去污因子为5.4×10~3;U的化学收率为96%,对U的去污因子为2.8×10~3。
It is required to separate uranium and protactinium in the determination of highly enriched uranium age.Distribution coefficients of uranium and protactinium were studied with the concentration of hydrochloric acid,hydrofluoric acid,and so on using nature uranium and 233 Pa as tracers.The method of separating protactinium and uranium using the TEVA chromatographic method was developed.The radiochemical recovery of protactinium is 99%.The decontamination factor for protactinium is 5.4×10 3.The chemical recovery rate of uranium is 96%,and the decontamination factor for uranium is 2.8×10 3.
作者
吴俊德
岳远振
杨磊
丁有钱
毛国淑
刘永利
刘耀阳
矫彩山
WU Jun-de;YUE Yuan-zhen;YANG Lei;DING You-qian;MAO Guo-shu;LIU Yong-li;LIU Yao-yang;JIAO Cai-shan(New Era Engineering Consulting Co.,Ltd.,Beijing 100088,China;;Department of Radiochemistry,China Institute of Atomic Energy,Beijing 102413,China;College of Nuclear Science and Technology,Harbin Engineering University,Harbin 150001,China)
出处
《核化学与放射化学》
CAS
CSCD
北大核心
2018年第5期290-293,共4页
Journal of Nuclear and Radiochemistry
关键词
PA
U
TEVA色层法
分离
Pa
U
TEVA chromatographic method
separation
