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氧化石墨烯对亚甲基蓝的可见光催化降解 被引量:4

Degradation of methylene blue by graphene oxide under visible-light irradiation
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摘要 用改良的Hummers法制得了氧化石墨烯,对其微观形貌、成分和结构进行了表征,并使用亚甲基蓝溶液测试其光催化效率。通过SEM、TEM、Raman分析表明,得到的是少层氧化石墨烯,碳氧原子数比在3∶1左右。荧光共聚焦光谱显示,所得到的氧化石墨烯在420~700nm的光波谱范围内都有特征吸收峰。氧化石墨烯能够迅速吸附亚甲基蓝分子,然后对其进行光催化降解,在亚甲基蓝浓度为40mg/L、氧化石墨烯浓度为10mg/L时,降解率能达到40%。之后,初步探究了氧化石墨烯的光催化机理。 The graphene oxide was prepared by modified Hummer method.Its microstructure,composition and structure were characterized and the photocatalytic efficiency was tested using methylene blue solution.SEM,TEM and raman analysis showed that few layer graphene oxide was obtained,and the ratio of carbon to oxygen was about 3∶1.Fluorescence confocal spectroscopy showed that the dispersion of graphene oxide had characteristic absorption peaks in the range of 420~700 nm.It was found that the methylene blue molecule was rapidly adsorbed then degraded by the graphene oxide under visible light.The degradation efficiency could reach 40%when the catalyst concentration was10 mg/L and the concentration of methylene blue was 40 mg/L.Its photocatalytic mechanism was also discussed then.
作者 刘洋洋 顾宝珊 郑艳银 梁东明 杨培燕 张启富 Liu Yangyang;Gu Baoshan;Zheng Yanyin;Liang Dongming;Yang Peiyan;Zhang Qifu(l.New Metallurgy High-Tech Group Co.,Ltd.,Beijing 100081;School of Materials Science andEngineering,Hebei University of Science & Technology,Shijiazhuang 050000)
出处 《化工新型材料》 CAS CSCD 北大核心 2019年第3期211-215,共5页 New Chemical Materials
关键词 氧化石墨烯 亚甲基蓝 可见光催化 羟基自由基 graphene oxide methylene blue visible-light catalysis hydroxyl radical
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