摘要
Due to the increasing environmental and energy issues, hydrogen, as a clean and non-carbon energy source, has received more and more attention in the past decades. Photocatalysis has been known as a promising approach for hydrogen generation and a key measure in solving serious environmental problems. Different from traditional catalysts, such as ZnO and TiO2, two-dimensional (2D) materials display unique advantages to hydrogen production due to their large specific surface area, high charge migration rate, tunable electronic structure and ultra-lightweight [1]. Especially, 2D materials show short migration distance for the generated electrons and holes, leading to the reduction of electron-hole recombination, which is one of the key factors affecting photocatalytic efficiency [2-4].
基金
supported by the National Natural Science Foundation of China (61625401, 61474033, and 61574050)
the Ministry of Science and Technology of China (2016YFA0200700)
Strategic Priority Research Program of the Chinese Academy of Sciences (XDA09040201)