摘要
Spin-dependent transport in ferromagnet/organic-ferromagnet/metal junctions is investigated theoretically.The results reveal a large tunneling magnetoresistance up to 3230%by controlling the relative magnetization orientation between the ferromagnet and the central organic ferromagnet.The mechanism is explained by distinct efficient spin-resolved tunneling states in the ferromagnet between the parallel and antiparallel spin configurations.The key role of the organic ferromagnet in generating the large magnetoresistance is explored,where the spin selection effect is found to enlarge the difference of the tunneling states between the parallel and antiparallel configurations by comparing with the conventional organic spin valves.The effects of intrinsic interactions in the organic ferromagnet including electron–lattice interaction and spin coupling with radicals on the magnetoresistance are discussed.This work demonstrates a promising potential of organic ferromagnets in the design of high-performance organic spin valves.
Spin-dependent transport in ferromagnet/organic-ferromagnet/metal junctions is investigated theoretically. The results reveal a large tunneling magnetoresistance up to 3230% by controlling the relative magnetization orientation between the ferromagnet and the central organic ferromagnet. The mechanism is explained by distinct efficient spin-resolved tunneling states in the ferromagnet between the parallel and antiparallel spin configurations. The key role of the organic ferromagnet in generating the large magnetoresistance is explored, where the spin selection effect is found to enlarge the difference of the tunneling states between the parallel and antiparallel configurations by comparing with the conventional organic spin valves. The effects of intrinsic interactions in the organic ferromagnet including electron–lattice interaction and spin coupling with radicals on the magnetoresistance are discussed. This work demonstrates a promising potential of organic ferromagnets in the design of high-performance organic spin valves.
作者
李彦琪
阚洪君
苗圆圆
杨磊
邱帅
张广平
任俊峰
王传奎
胡贵超
Yan-Qi Li;Hong-Jun Kan;Yuan-Yuan Miao;Lei Yang;Shuai Qiu;Guang-Ping Zhang;Jun-Feng Ren;Chuan-Kui Wang;Gui-Chao Hu(Shandong Province Key Laboratory of Medical Physics and Image Processing Technology,School of Physics and Electronics,Shandong Normal University,Jinan 250100,China)
基金
Project supported by the National Natural Science Foundation of China(Grant Nos.11974215,11704230,11674197,and 11874242)
the Natural Science Foundation of Shandong Province,China(Grant No.ZR2019MA043)
the Taishan Scholar Project of Shandong Province,China