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Nitrogen and sulfur co-doped graphene aerogel with hierarchically porous structure for high-performance supercapacitors 被引量:6

Nitrogen and sulfur co-doped graphene aerogel with hierarchically porous structure for high-performance supercapacitors
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摘要 Supercapacitors with unique performance have been widely utilized in many fields. Herein, we report a nitrogen and sulfur co-doped graphene aerogel(N/S-GA-2) prepared using a low toxic precursor for high-performance supercapacitors. The as-obtained material possesses a hierarchically porous structure and a large number of electrochemical active sites. At a current density of 1 Ag^-1, the specific capacitance of the N/S-GA-2 for supercapacitors with the ionic liquid as the electrolyte is 169.4 Fg^-1, and the corresponding energy density is 84.5 Wh kg^-1.At a power density of 8.9 k W kg^-1, the energy density can reach up to 75.7 Wh kg^-1, showing that the N/S-GA-2 has an excellent electrochemical performance. Consequently, the N/S-GA-2 can be used as a promising candidate of electrode materials for supercapacitors with high power density and high energy density. Supercapacitors with unique performance have been widely utilized in many fields. Herein, we report a nitrogen and sulfur co-doped graphene aerogel(N/S-GA-2) prepared using a low toxic precursor for high-performance supercapacitors. The as-obtained material possesses a hierarchically porous structure and a large number of electrochemical active sites. At a current density of 1 A g-1, the specific capacitance of the N/S-GA-2 for supercapacitors with the ionic liquid as the electrolyte is 169.4 F g-1, and the corresponding energy density is 84.5 Wh kg-1.At a power density of 8.9 k W kg-1, the energy density can reach up to 75.7 Wh kg-1, showing that the N/S-GA-2 has an excellent electrochemical performance. Consequently, the N/S-GA-2 can be used as a promising candidate of electrode materials for supercapacitors with high power density and high energy density.
出处 《Green Energy & Environment》 CSCD 2020年第1期69-75,共7页 绿色能源与环境(英文版)
基金 Financial support from the National Natural Science Foundation of China (Nos. 21873026 and 21573058) the Program for Innovative Research Team in Science and Technology in University of Henan Province (17IRTSTHN 001) is gratefully acknowledged
关键词 Graphene aerogel Hierarchically porous structure SUPERCAPACITOR Ionic liquid Graphene aerogel Hierarchically porous structure Supercapacitor Ionic liquid
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