摘要
本研究基于2015年在线监测等数据,分析中国钢铁行业主要工序(烧结和球团)排口烟气浓度情况,自下而上建立了2015年中国高时空分辨率钢铁行业大气污染物排放清单(HSEC, 2015),使用CAMx模型,定量模拟钢铁行业排放对区域大气污染物浓度贡献.结果表明, 2015年中国钢铁行业共排放SO2、NOx、PM10、PM2.5、PCDD/Fs、VOCs、CO、BC、OC、EC和F分别为37.48万t、 72.05万t、 33.48万t、 15.03万t、 1.91 kg、 84.29万t、 3 478.85万t、 0.64万t、 0.83万t、 0.08万t和0.77万t.从区域角度:上海和天津钢铁行业单位面积污染排放强度最大,对区域大气污染贡献比例较高.从工序角度:2015年烧结和球团烟气排口月平均浓度降低.从污染物角度:2015年钢铁行业排放NOx对区域污染物浓度贡献最大,NOx具有较大的减排潜力.
Based on the data from a continuous emission monitoring systems network in 2015,this study analyzed the compliance rates of exhaust gas in the processes of China's iron and steel industry,and established a high-resolution steel plant emission inventory for China(HSEC,2015),based on the bottom-up method.The contribution of emissions from the iron and steel industry to regional air quality was quantitatively simulated using a CAMx model.The results showed that in 2015,the total emissions of SO2,NOx,PM10,PM2.5,PCDD/Fs,VOCs,CO,BC,OC,EC,and F were 374800 t,720500 t,334800 t,150300 t,1.91 kg,842900 t,34788500 t,6400 t,8300 t,800 t,and 7700 t,respectively.From a regional perspective,the iron and steel industry in Shanghai and Tianjin has the highest emission intensity per unit area and contributes a high proportion to regional air pollution.From a process perspective,in 2015,the exhaust concentration of flue gas in the main process gradually decreased,with a high compliance rate,and the emission factor significantly decreased to lower than that in the existing research results.From a species perspective,in 2015,NOx emission from the steel industry contributed the most to regional air quality,and there is therefore a great emission reduction potential for NOx.
作者
汤铃
薛晓达
伯鑫
贾敏
郭静
田军
黄满堂
崔维庚
王彤
李时蓓
敬红
甄瑞卿
孙露
成国庆
TANG Ling;XUE Xiao-da;BO Xin;JIA Min;GUO Jing;TIAN Jun;HUANG Man-tang;CUI Wei-geng;WANG Tong;LI Shi-bei;JING Hong;ZHEN Rui-qing;SUN Lu;CHENG Guo-qing(School of Economics and Management,Beihang University,Beijing 100191,China;School of Economics and Management,Beijing University of Chemical Technology,Beijing 100029,China;Appraisal Centre for Environment and Engineering,Ministry of Ecology and Environment,Beijing 100012,China;Academy of Environmental Planning&Design,Co.,Ltd.,Nanjing University,Nanjing 210093,China;School of Earth Sciences and Resources,Chang'an University,Xi'an 710054,China;Shaanxi Environmental Investigation and Assessment Center,Xi'an 710000,China;China National Environmental Monitoring Centre,Beijing 100012,China;MCC Capital Engineering&Research Incorporation Limited,Beijing 100176,China;Center for Social and Environmental Systems Research,National Institute for Environmental Studies,Ibaraki 305-8506,Japan;Hebei Zhengrun Environmental Technology Co.,Ltd.,Shijiazhuang 050091,China)
出处
《环境科学》
EI
CAS
CSCD
北大核心
2020年第7期2981-2994,共14页
Environmental Science
基金
国家重点实验室开放基金项目(16K01ESPCT)
国家重点研发计划项目(2016YFC0208101,2017YFC0210300)
大气重污染成因与治理攻关项目(DQGG0209-07,DQGG0304-07)
生态环境部环境工程评估中心创新科研项目(2019-10)
国家自然科学基金项目(71971007,71622011)。
关键词
排放清单
钢铁
大气污染
CAMx模型
排放因子
emission inventory
iron and steel
air pollution
CAMx model
emission factor