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Visible-light induced generation of bifunctional nitrogen-centered radicals:a concise synthetic strategy to construct bicyclo[3.2.1]octane and azepane cores 被引量:1

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摘要 A photocatalytic tandem cyclization of o-alkenylbenzaldehydes using pyridinium salts as the amination reagent is described.A variety of valuable seven-membered nitrogenous heterocyclic skeletons are prepared in modest to excellent yields in concise one-step.This transformation features mild reaction conditions and exceptional functional group tolerance.In addition,combining control experiments and density functional theory(DFT)calculations on the mechanism can explain the reaction selectivity.
出处 《Science China Chemistry》 SCIE EI CAS CSCD 2021年第2期274-280,共7页 中国科学(化学英文版)
基金 the National Natural Science Foundation of China(21632003,21871116) the Key Program of Gansu Province(17ZD2GC011) the‘‘111’’Program from the MOE of China。
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