摘要
Oxygen reduction reaction (ORR) is an important process for the conversion and utilization of a wide range of renewable energy sources, and is critical for the shape of future energy scenario [1–10]. However, ORR is a complex four-electron transfer process and is kinetically sluggish. It is urgent to develop high-efficient electrocatalysts to solve this problem [11–15]. Up to now, precious metal-based catalysts such as Pt-based electrocatalysts have been widely studied and found to be one of the most efficient electrocatalysts for ORR. However, the high price and the small reserves limit their large-scale commercialization [10,16–23]. Therefore, in order to fulfill needs for the practical applications, it is necessary to develop low-cost electrocatalysts, also with high activity and great stability [19,24–28].
基金
supported by the National Natural Science Foundation of China(Grant No.21975148,21601118,21773146,21902099,and 21905167)
the Fundamental Research Funds for the Central Universities(GK201903033 and GK202003025)
the “Thousand Talents Program”of China
the Fok Ying-Tong Education Foundation for Outstanding Young Teachers in University
the China Postdoctoral Science Foundation(2019M650254,and 2020T130391)
the Opening Fund of State Key Laboratory of Heavy Oil Processing(SKLOP202002005)
the Research Fund Program of Key Laboratory of Fuel Cell Technology of Guangdong Province
the Research Funds of Shaanxi Normal University。