摘要
Based on the time-dependent theory, an analysis of the distinction between resonance Raman (RR) and resonance fluorescence (RF) with pulse excitation was presented. The real population of the intermediate state gives two optical components-the independent time evolution of intermediate ket and bra states generates RR while RF originates from the phase coherent between ket and bra states. In cw limit, the transition probability of spontaneous emission with pulse excitation can be reduced to the classical theory.
作者
LU Jing
DU Si-De
FAN Kang-Nian
Lee Soo-Ying
陆靖;杜四德;范康年;Lee Soo-Ying(Department of Chemistry,Fudan University,Shanghai 200433;Department of Physics,Fudan University,Shanghai 200433;Department of Chemistry,National University of Singapore,Singapore 119260,Singapore)
基金
Supported by the National Natural Science Foundation of China under Grant Nos.29773010 and 29833080。
